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With the demonstration of quantum-limited optical time transfer capable of tolerating the losses associated with long ground-to-space links, two future applications of free-space time transfer have emerged: intercontinental clock comparisons for time dissemination and coherence transfer for future distributed sensing in the mm-wave region. In this paper, we estimated the projected performance of these two applications using quantum-limited optical time transfer and assuming existing low-size, low-weight, and low-power hardware. In both cases, we limit the discussion to the simplest case of a single geosynchronous satellite linked to either one or two ground stations. One important consideration for such future space-based operations is the choice of reference oscillator onboard the satellite. We find that with a modestly performing optical reference oscillator and low-power fiber-based frequency combs, quantum-limited time transfer could support intercontinental clock comparisons through a common-view node in geostationary orbit with a modified Allan deviation at the 10−16 level at 10-s averaging time, limited primarily by residual turbulence piston noise. In the second application of coherence transfer from ground-to-geosynchronous orbit, we find the system should support high short-term coherence with ∼10 millirad phase noise on a 300 GHz carrier at essentially unlimited integration times. 

We configure a fiber-laser based dual-comb spectrometer to measure the O2 delta band (1260 nm) in addition to CO2 and CH4 absorption features (1600 nm). 

To better quantify methane emissions resulting from grazing cattle, a controlled methane release at an agricultural site is performed using dual comb spectroscopy. The achieved methane concentration precision is below 10 nmol/mol. The Author(s) Work of the US Government and not subject to copyright. 

Advances in spectroscopy have the potential to improve our understanding of agricultural processes and associated trace gas emissions. We implement field-deployed, open-path dual-comb spectroscopy (DCS) for precise multispecies emissions estimation from livestock. With broad atmospheric dual-comb spectra, we interrogate upwind and downwind paths from pens containing approximately 300 head of cattle, providing time-resolved concentration enhancements and fluxes of CH 4 , NH 3 , CO 2 , and H 2 O. The methane fluxes determined from DCS data and fluxes obtained with a colocated closed-path cavity ring-down spectroscopy gas analyzer agree to within 6%. The NH 3 concentration retrievals have sensitivity of 10 parts per billion and yield corresponding NH3 fluxes with a statistical precision of 8% and low systematic uncertainty. Open-path DCS offers accurate multispecies agricultural gas flux quantification without external calibration and is easily extended to larger agricultural systems where point-sampling-based approaches are insufficient, presenting opportunities for field-scale biogeochemical studies and ecological monitoring.