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Abstract We report the discovery of a new subclass of carbon-enhanced metal-poor (CEMP) stars, characterized by high absolute carbon abundances (A(C) > 7.39) and extremely low metallicity ([Fe/H] ≤ –3.1) but notably lacking enhancements in neutron-capture elements, thus falling under the CEMP-no category. This population emerged from a detailed analysis of low-resolution spectroscopic data obtained from the Sloan Digital Sky Survey and the Large Sky Area Multi-Object Fiber Spectroscopic Telescope, where the observed frequency trends with the decreasing metallicity of CEMP-s(s-process-enhanced) and CEMP-no (no neutron-capture enhanced) stars deviated from established expectations. In contrast to earlier findings, we observe a rise in high-A(C) stars below [Fe/H] = −3.1, which we interpret as a distinct group not accounted for in traditional CEMP classifications. Following the Yoon–Beers group classification, we define these stars as Group IV. Statistical modeling confirms their presence as a separate peak in theA(C) distribution, and available radial velocity data suggest that about 30% of Group IV stars may be binaries, indicating possible binary-related formation mechanisms. This discovery challenges the current CEMP-no star formation pathways and implies the existence of alternative or hybrid enrichment scenarios in the early Universe. High-resolution spectroscopic follow-up of Group IV candidates will be crucial for identifying their progenitors and understanding their evolutionary implications.