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Abstract Many problems in fluid mechanics require single-shot 3D measurements of fluid flows, but are limited by available techniques. Here, we design and build a novel flexible high-speed two-color scanning volumetric laser-induced fluorescence (H2C-SVLIF) technique. The technique is readily adaptable to a range of temporal and spatial resolutions, rendering it easily applicable to a wide spectrum of experiments. The core equipment consists of a single monochrome high-speed camera and a pair of ND: YAG lasers pulsing at different wavelengths. The use of a single camera for direct 3D imaging eliminates the need for complex volume reconstruction algorithms and easily allows for the correction of distortion defects. Motivated by the large data loads that result from high-speed imaging techniques, we develop a custom, open-source, software package, which allows for real time playback with correction of perspective defects while simultaneously overlaying arbitrary 3D data. The technique is capable of simultaneous measurement of 3D velocity fields and a secondary tracer in the flow. To showcase the flexibility and adaptability of our technique, we present a set of experiments: (1) the flow past a sphere, and (2) vortices embedded in laminar pipe flow. In the first experiment, two channel measurements are taken at a resolution of 512 × 512 × 512 with volume rates of 65.1 Hz. In the second experiment, a single-color SVLIF system is integrated on a moving stage, providing imaging at 1280 × 304 × 256 with volume rates of 34.8 Hz. Although this second experiment is only single channel, it uses identical software and much of the same hardware to demonstrate the extraction of multiple information channels from single channel volumetric images. 

We study the effects of the optical binding force on wavelength sized colloidal particles free to move in a counter-propagating beam. This work is motivated by the concept of using optical binding to direct the assembly of large numbers of colloidal particles; previous work has used small numbers of particles and/or 1D or 2D restricted geometries. Utilizing a novel experimental scheme, we describe the general static and dynamic self-organization behaviors for 20–100 particles free to move in 3-dimensional space. We observe the self-organization of the colloids into large optically bound structures along with the formation of driven particle clusters. Furthermore we show that the structure and behavior of these optically bound systems can be tuned using the refractive index of the particles and properties of the binding light. In particular, we show that the driven behavior originates from N -body interactions, which has significant implications for future work on optically bound clusters of more than 2 particles. 

For magnetite spherical nanoparticles, the orientation of the dipole moment in the crystal does not affect the morphology of either zero field or field induced structures. For non-spherical particles however, an interplay between particle shape and direction of the magnetic moment can give rise to unusual behaviors, in particular when the moment is not aligned along a particle symmetry axis. Here we disclose for the first time the unique magnetic properties of hematite cubic particles and show the exact orientation of the cubes' dipole moment. Using a combination of experiments and computer simulations, we show that dipolar hematite cubes self-organize into dipolar chains with morphologies remarkably different from those of spheres, and demonstrate that the emergence of these structures is driven by competing anisotropic interactions caused by the particles' shape anisotropy and their fixed dipole moment. Furthermore, we have analytically identified a specific interplay between energy, and entropy at the microscopic level and found that an unorthodox entropic contribution mediates the organization of particles into the kinked nature of the dipolar chains.