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Understanding the nature of high-redshift dusty galaxies requires a comprehensive view of their interstellar medium (ISM) and molecular complexity. However, the molecular ISM at high redshifts is commonly studied using only a few species beyond¹²C¹⁶O, limiting our understanding. In this paper, we present the results of deep 3 mm spectral line surveys using the NOrthern Extended Millimeter Array (NOEMA) targeting two strongly lensed dusty galaxies observed when the Universe was less than 1.8 Gyr old: APM 08279+5255, a quasar at redshiftz= 3.911, and NCv1.143 (H-ATLAS J125632.7+233625), az= 3.565 starburst galaxy. The spectral line surveys cover rest-frame frequencies from about 330 to 550 GHz for both galaxies. We report the detection of 38 and 25 emission lines in APM 08279+5255 and NCv1.143, respectively. These lines originate from 17 species, namely CO,¹³CO, C¹⁸O, CN, CCH, HCN, HCO⁺, HNC, CS, C³⁴S, H₂O, H₃O⁺, NO, N₂H⁺, CH, c-C₃H₂, and the vibrationally excited HCN and neutral carbon. The spectra reveal the chemical richness and the complexity of the physical properties of the ISM. By comparing the spectra of the two sources and combining the analysis of the molecular gas excitation, we find that the physical properties and the chemical imprints of the ISM are different: the molecular gas is more excited in APM 08279+5255, which exhibits higher molecular gas temperatures and densities compared to NCv1.143; the molecular abundances in APM 08279+5255 are akin to the values of local active galactic nuclei (AGN), showing boosted relative abundances of the dense gas tracers that might be related to high-temperature chemistry and/or the X-ray-dominated regions, while NCv1.143 more closely resembles local starburst galaxies. The most significant differences between the two sources are found in H₂O: the 448 GHz ortho-H₂O(4₂₃ − 3₃₀) line is significantly brighter in APM 08279+5255, which is likely linked to the intense far-infrared radiation from the dust powered by AGN. Our astrochemical model suggests that, at such high column densities, far-ultraviolet radiation is less important in regulating the ISM, while cosmic rays (and/or X-rays and shocks) are the key players in shaping the molecular abundances and the initial conditions of star formation. Both our observed CO isotopologs line ratios and the derived extreme ISM conditions (high gas temperatures, densities, and cosmic-ray ionization rates) suggest the presence of a top-heavy stellar initial mass function. From the ∼330–550 GHz continuum, we also find evidence of nonthermal millimeter flux excess in APM 08279+5255 that might be related to the central supermassive black hole. Such deep spectral line surveys open a new window into the physics and chemistry of the ISM and the radiation field of galaxies in the early Universe. 

Abstract The Dragonfly galaxy (MRC 0152-209), the most infrared-luminous radio galaxy at redshiftz∼ 2, is a merger system containing a powerful radio source and large displacements of gas. We present kiloparsec-resolution data from the Atacama Large Millimeter/submillimeter Array and the Very Large Array of carbon monoxide (6−5), dust, and synchrotron continuum, combined with Keck integral field spectroscopy. We find that the Dragonfly consists of two galaxies with rotating disks that are in the early phase of merging. The radio jet originates from the northern galaxy and brightens when it hits the disk of the southern galaxy. The Dragonfly galaxy therefore likely appears as a powerful radio galaxy because its flux is boosted into the regime of high-zradio galaxies by the jet–disk interaction. We also find a molecular outflow of (1100 ± 550)M_⊙yr⁻¹associated with the radio host galaxy, but not with the radio hot spot or southern galaxy, which is the galaxy that hosts the bulk of the star formation. Gravitational effects of the merger drive a slower and longer-lived mass displacement at a rate of (170 ± 40)M_⊙yr⁻¹, but this tidal debris contains at least as much molecular gas mass as the much faster outflow, namelyM_H2= (3 ± 1) × 10⁹(α_CO/0.8)M_⊙. This suggests that both the active-galactic-nucleus-driven outflow and mass transfer due to tidal effects are important in the evolution of the Dragonfly system. The Keck data show Lyαemission spread across 100 kpc, and Civand Heiiemission across 35 kpc, confirming the presence of a metal-rich and extended circumgalactic medium previously detected in CO(1–0).