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Free, publicly-accessible full text available May 1, 2023
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Free, publicly-accessible full text available February 1, 2023
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Free, publicly-accessible full text available December 1, 2022
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Thermoelectric (TE) cement composite is a new type of TE material. Unlike ordinary cement, TE cement can mutually convert thermal energy to electrical energy due to the addition of carbon fibers, metal oxide nanoparticles, etc. In hot summer or cold winter, the significant temperature difference between indoor and outdoor can be used by TE cement to generate electricity. On the other hand, given power input, the same material can provide cooling/ heating to adjust room temperature. Therefore, TE cement has certain energy-saving potential in the application of building enclosures and energy systems. Its ability to convert different forms of energymore »
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Free, publicly-accessible full text available September 1, 2022
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Single-atom catalysts (SACs) exhibit unique catalytic property and maximum atom efficiency of rare, expensive metals. A critical barrier to applications of SACs is sintering of active metal atoms under operating conditions. Anchoring metal atoms onto oxide supports via strong metal-support bonds may alleviate sintering. Such an approach, however, usually comes at a cost: stabilization results from passivation of metal sites by excessive oxygen ligation—too many open coordination sites taken up by the support, too few left for catalytic action. Furthermore, when such stabilized metal atoms are activated by reduction at elevated temperatures they become unlinked and so move and sinter,more »
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Free, publicly-accessible full text available February 1, 2023
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Sc 3 Mn 3 Al 7 Si 5 is a rare example of a correlated metal in which the Mn moments form a kagome lattice. The absence of magnetic ordering to the lowest temperatures suggests that geometrical frustration of magnetic interactions may lead to strong magnetic fluctuations. We have performed inelastic neutron scattering measurements on Sc 3 Mn 3 Al 7 Si 5 , finding that phonon scattering dominates for energies from ∼20–50 meV. These results are in good agreement with ab initio calculations of the phonon dispersions and densities of states, and as well reproduce the measured specific heat.more »Free, publicly-accessible full text available October 12, 2022