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We search for dark matter in the form of axionlike particles (ALPs) in the mass range by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHZ resulted in a sensitivity to the ALP-proton coupling constant of . This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment’s capabilities. CASPEr-Gradient Low-Field will probe the mass range from to with hyperpolarized samples to boost the sensitivity beyond the astronomical limits.more » « lessFree, publicly-accessible full text available September 1, 2026
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