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Creators/Authors contains: "Masson, E."

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  1. ; ; ; ; ; ; ; ; ; ; et al ( , Journal of Instrumentation)
    Abstract Understanding propagation of scintillation light is critical for maximizing the discovery potential of next-generation liquid xenon detectors that use dual-phase time projection chamber technology. This work describes a detailed optical simulation of the DARWIN detector implemented using Chroma, a GPU-based photon tracking framework. To evaluate the framework and to explore ways of maximizing efficiency and minimizing the time of light collection, we simulate several variations of the conventional detector design. Results of these selected studies are presented. More generally, we conclude that the approach used in this work allows one to investigate alternative designs faster and in more detailmore »than using conventional Geant4 optical simulations, making it an attractive tool to guide the development of the ultimate liquid xenon observatory.« less
    Free, publicly-accessible full text available July 1, 2023
  2. ; ; ; ; ; ; ; ( , Chemical science)
    A series of molecular rotors was designed to study and measure the rate accelerating effects of an intramolecular hydrogen bond. The rotors form a weak neutral O–H/O]C hydrogen bond in the planar transition state (TS) of the bond rotation process. The rotational barrier of the hydrogen bonding rotors was dramatically lower (9.9 kcal mol1) than control rotors which could not form hydrogen bonds. The magnitude of the stabilization was significantly larger than predicted based on the independently measured strength of a similar OH/OC hydrogen bond (1.5 kcal mol-1). The origins of the large transition state stabilization were studied via experimentalmore »substituent effect and computational perturbation analyses. Energy decomposition analysis of the hydrogen bonding interaction revealed a significant reduction in the repulsive component of the hydrogen bonding interaction. The rigid framework of the molecular rotors positions and preorganizes the interacting groups in the transition state. This study demonstrates that with proper design a single hydrogen bond can lead to a TS stabilization that is greater than the intrinsic interaction energy, which has applications in catalyst design and in the study of enzyme mechanisms.« less
    Accepted Manuscript Full Text Available
  3. ; ; ; ; ; ; ; ; ; ; et al ( , The European Physical Journal C)
    Abstract The selection of low-radioactive construction materials is of the utmost importance for rare-event searches and thus critical to the XENONnT experiment. Results of an extensive radioassay program are reported, in which material samples have been screened with gamma-ray spectroscopy, mass spectrometry, and $$^{222}$$ 222 Rn emanation measurements. Furthermore, the cleanliness procedures applied to remove or mitigate surface contamination of detector materials are described. Screening results, used as inputs for a XENONnT Monte Carlo simulation, predict a reduction of materials background ( $$\sim $$ ∼ 17%) with respect to its predecessor XENON1T. Through radon emanation measurements, the expected $$^{222}$$ 222more »Rn activity concentration in XENONnT is determined to be 4.2 ( $$^{+0.5}_{-0.7}$$ - 0.7 + 0.5 )  $$\upmu $$ μ Bq/kg, a factor three lower with respect to XENON1T. This radon concentration will be further suppressed by means of the novel radon distillation system.« less
    Free, publicly-accessible full text available July 1, 2023
  4. ; ; ; ; ; ; ; ; ; ; et al ( , Physical Review D)
    Free, publicly-accessible full text available July 1, 2023
  5. ; ; ; ; ; ; ; ; ; ; et al ( , Progress of Theoretical and Experimental Physics)
    Abstract A novel online distillation technique was developed for the XENON1T dark matter experiment to reduce intrinsic background components more volatile than xenon, such as krypton or argon, while the detector was operating. The method is based on a continuous purification of the gaseous volume of the detector system using the XENON1T cryogenic distillation column. A krypton-in-xenon concentration of (360±60)ppq was achieved. It is the lowest concentration measured in the fiducial volume of an operating dark matter detector to date. A model was developed and fit to the data to describe the krypton evolution in the liquid and gas volumesmore »of the detector system for several operation modes over the time span of 550 days, including the commissioning and science runs of XENON1T. The online distillation was also successfully applied to remove 37Ar after its injection for a low energy calibration in XENON1T. This makes the usage of 37Ar as a regular calibration source possible in the future. The online distillation can be applied to next-generation LXe TPC experiments to remove krypton prior to, or during, any science run. The model developed here allows further optimization of the distillation strategy for future large scale detectors.« less
    Free, publicly-accessible full text available April 29, 2023
  6. ; ; ; ; ; ; ; ; ; ; et al ( , The European Physical Journal C)
    Abstract The DARWIN observatory is a proposed next-generation experiment to search for particle dark matter and for the neutrinoless double beta decay of $$^{136}$$ 136 Xe. Out of its 50 t total natural xenon inventory, 40 t will be the active target of a time projection chamber which thus contains about 3.6 t of $$^{136}$$ 136 Xe. Here, we show that its projected half-life sensitivity is $$2.4\times {10}^{27}\,{\hbox {year}}$$ 2.4 × 10 27 year , using a fiducial volume of 5 t of natural xenon and 10 year of operation with a background rate of less than 0.2 events/(t  $$\cdot $$ ·  year) in the energymore »region of interest. This sensitivity is based on a detailed Monte Carlo simulation study of the background and event topologies in the large, homogeneous target. DARWIN will be comparable in its science reach to dedicated double beta decay experiments using xenon enriched in $$^{136}$$ 136 Xe.« less
    Full Text Available 
  7. ; ; ; ; ; ; ; ; ; ; et al ( , The European Physical Journal C)
    Abstract We detail the sensitivity of the proposed liquid xenon DARWIN observatory to solar neutrinos via elastic electron scattering. We find that DARWIN will have the potential to measure the fluxes of five solar neutrino components: pp , $$^7$$ 7 Be, $$^{13}$$ 13 N, $$^{15}$$ 15 O and pep . The precision of the $$^{13}$$ 13 N, $$^{15}$$ 15 O and pep components is hindered by the double-beta decay of $$^{136}$$ 136 Xe and, thus, would benefit from a depleted target. A high-statistics observation of pp neutrinos would allow us to infer the values of the electroweak mixing angle, $$\sinmore »^2\theta _w$$ sin 2 θ w , and the electron-type neutrino survival probability, $$P_{ee}$$ P ee , in the electron recoil energy region from a few keV up to 200 keV for the first time, with relative precision of 5% and 4%, respectively, with 10 live years of data and a 30 tonne fiducial volume. An observation of pp and $$^7$$ 7 Be neutrinos would constrain the neutrino-inferred solar luminosity down to 0.2%. A combination of all flux measurements would distinguish between the high- (GS98) and low-metallicity (AGS09) solar models with 2.1–2.5 $$\sigma $$ σ significance, independent of external measurements from other experiments or a measurement of $$^8$$ 8 B neutrinos through coherent elastic neutrino-nucleus scattering in DARWIN. Finally, we demonstrate that with a depleted target DARWIN may be sensitive to the neutrino capture process of $$^{131}$$ 131 Xe.« less
    Full Text Available 
  8. ; ; ; ; ; ; ; ; ; ; et al ( , Physical Review Letters)
    Full Text Available 
  9. ; ; ; ; ; ; ; ; ; ; et al ( , Physical Review C)
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  10. ; ; ; ; ; ; ; ; ; ; et al ( , Physics Letters B)
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