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We present a novel methodology for crafting effective public messages by combining large language models (LLMs) and conjoint analysis. Our approach personalizes messages for diverse personas – context-specific archetypes representing distinct attitudes and behaviors – while reducing the costs and time associated with traditional surveys. We tested this method in public health contexts (e.g., COVID-19 mandates) and civic engagement initiatives (e.g., voting). A total of 153 distinct messages were generated, each composed of components with varying levels, and evaluated across five personas tailored to each context. Conjoint analysis identified the most effective message components for each persona, validated through a study with 2,040 human participants. This research highlights LLMs’ potential to enhance public communication, providing a scalable, cost-effective alternative to surveys, and offers new directions for HCI, particularly for the design of adaptive, user-centered, persona-driven interfaces and systems.