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We study the 3.4 − 4.4 μm fundamental rovibrational band of H₃⁺, a key tracer of the ionization of the molecular interstellar medium (ISM), in a sample of 12 local (d < 400 Mpc) (ultra)luminous infrared galaxies ((U)LIRGs) observed with JWST/NIRSpec. TheP,Q, andRbranches of the band are detected in 13 out of 20 analyzed regions within these (U)LIRGs, which increases the number of extragalactic H₃⁺detections by a factor of 6. For the first time in the ISM, the H₃⁺band is observed in emission; we detect this emission in three regions. In the remaining ten regions, the band is seen in absorption. The absorptions are produced toward the 3.4 − 4.4 μm hot dust continuum rather than toward the stellar continuum, indicating that they likely originate in clouds associated with the dust continuum source. The H₃⁺band is undetected in Seyfert-like (U)LIRGs where the mildly obscured X-ray radiation from the active galactic nuclei might limit the abundance of this molecule. For the detections, the H₃⁺abundances,N(H₃⁺)/N_H = (0.5 − 5.5)×10⁻⁷, imply relatively high ionization rates,ζ_H2, of between 3 × 10⁻¹⁶and > 4 × 10⁻¹⁵s⁻¹, which are likely associated with high-energy cosmic rays. In half of the targets, the absorptions are blueshifted by 50–180 km s⁻¹, which is lower than the molecular outflow velocities measured using other tracers such as OH 119 μm or rotational CO lines. This suggests that H₃⁺traces gas close to the outflow-launching sites before it has been fully accelerated. We used nonlocal thermodynamic equilibrium models to investigate the physical conditions of these clouds. In seven out of ten objects, the H₃⁺excitation is consistent with inelastic collisions with H₂in warm translucent molecular clouds (T_kin ∼ 250–500 K andn(H₂) ∼10^2 − 3cm⁻³). In three objects, dominant infrared pumping excitation is required to explain the absorptions from the (3,0) and (2,1) levels of H₃⁺detected for the first time in the ISM. 

Abstract We report new observations toward the hyperluminous dusty starbursting major merger ADFS-27 ( z  = 5.655), using the Australia Telescope Compact Array (ATCA) and the Atacama Large Millimeter/submillimeter Array (ALMA). We detect CO ( J  = 2 → 1), CO ( J  = 8 → 7), CO ( J  = 9 → 8), CO ( J  = 10 → 9), and H 2 O (3 12  → 2 21 ) emission, and a P Cygni−shaped OH + (1 1  → 0 1 ) absorption/emission feature. We also tentatively detect H 2 O (3 21  → 3 12 ) and OH + (1 2 → 0 1 ) emission and CH + ( J  = 1 → 0) absorption. We find a total cold molecular mass of M gas  = (2.1 ± 0.2) × 10 11 ( α CO /1.0) M ⊙ . We also find that the excitation of the star-forming gas is overall moderate for a z > 5 dusty starburst, which is consistent with its moderate dust temperature. A high-density, high kinetic temperature gas component embedded in the gas reservoir is required to fully explain the CO line ladder. This component is likely associated with the “maximum starburst” nuclei in the two merging galaxies, which are separated by only 140 ± 13 km s −1 along the line of sight and 9.0 kpc in projection. The kinematic structure of both components is consistent with galaxy disks, but this interpretation remains limited by the spatial resolution of the current data. The OH + features are only detected toward the northern component, which is also the one that is more enshrouded in dust and thus remains undetected up to 1.6 μ m even in our sensitive new Hubble Space Telescope Wide Field Camera 3 imaging. The absorption component of the OH + line is blueshifted and peaks near the CO and continuum emission peak, while the emission is redshifted and peaks offset by 1.7 kpc from the CO and continuum emission peak, suggesting that the gas is associated with a massive molecular outflow from the intensely star-forming nucleus that supplies 125 M ⊙ yr −1 of enriched gas to its halo.