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Abstract Polarimetric data provide key insights into infrared emission mechanisms in the inner disks of young stellar objects (YSOs) and the details of dust formation around asymptotic giant branch (AGB) stars. While polarization measurements are well-established in radio interferometry, they remain challenging at visible and near-infrared wavelengths, due to the significant time-variable birefringence introduced by the complex optical beam train. In this study, we characterize instrumental polarization effects within the optical path of the Center for High Angular Resolution Astronomy (CHARA) Array, focusing on theH-band MIRC-X andK-band MYSTIC beam combiners. Using the Jones matrix formalism, we developed a comprehensive model describing diattenuation and retardance across the array. By applying this model to an unpolarized calibrator, we derived the instrumental parameters for both MIRC-X and MYSTIC. Our results show differential diattenuation consistent with ≥97% reflectivity per aluminum-coated surface at 45° incidence. The differential retardance exhibits small wavelength-dependent variations, in some cases larger than we expected. Notably, telescope W2 exhibits a significantly larger phase shift in the Coudé path, attributable to a fixed aluminum mirror (M4) used in place of deformable mirrors present on the other telescopes during the observing run. We also identify misalignments in the LiNbO₃birefringent compensator plates on S1 (MIRC-X) and W2 (MYSTIC). After correcting for night-to-night offsets, we achieve calibration accuracies of ±3.4% in visibility ratio and $\pm 1\stackrel{°}{.}4$in differential phase for MIRC-X, and ±5.9% and $\pm 2\stackrel{°}{.}4$, respectively, for MYSTIC. Given that the differential intrinsic polarization of spatially resolved sources, such as AGB stars and YSOs, typically greater than these instrumental uncertainties, our results demonstrate that CHARA is now capable of achieving high-accuracy measurements of intrinsic polarization in astrophysical targets.