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Creators/Authors contains: "Stein, Robin S."

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  1. ; ; ; ; ; ; (, Chemistry – A European Journal)
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  2. ; ; ; ; ; ; (, ChemRxiv)
    Mechanochemistry reveals a novel polymorph of the mercury(II) imidazolate framework, based on square-grid (sql) topology layers. Reaction monitoring and periodic density functional theory calculations show that the sql-structure is of higher stability than the previously reported three-dimensional framework, with the unexpected stabilization of the lower dimensionality structure arising from weak interactions that include short interlayer C-H···Hg contacts, highlighting a potential role for agostic interactions in directing metal-organic framework topology. 
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