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Atmospheric conditions affect the release of anemophilous pollen, and the timing and magnitude will be altered by climate change. As simulated with a pollen emission model and future climate data, warmer end-of-century temperatures (4–6 K) shift the start of spring emissions 10–40 days earlier and summer/fall weeds and grasses 5–15 days later and lengthen the season duration. Phenological shifts depend on the temperature response of individual taxa, with convergence in some regions and divergence in others. Temperature and precipitation alter daily pollen emission maxima by −35 to 40% and increase the annual total pollen emission by 16–40% due to changes in phenology and temperature-driven pollen production. Increasing atmospheric CO₂may increase pollen production, and doubling production in conjunction with climate increases end-of-century emissions up to 200%. Land cover change modifies the distribution of pollen emitters, yet the effects are relatively small (<10%) compared to climate or CO₂. These simulations indicate that increasing pollen and longer seasons will increase the likelihood of seasonal allergies.

 

The land surface hydrology of the North American Great Lakes region regulates ecosystem water availability, lake levels, vegetation dynamics, and agricultural practices. In this study, we analyze the Great Lakes terrestrial water budget using the Noah‐MP land surface model to characterize the catchment hydrological regimes and identify the dominant quantities contributing to the variability in the land surface hydrology. We show that the Great Lakes domain is not hydrologically uniform and strong spatiotemporal differences exist in the regulators of the hydrological budget at daily, monthly, and annual timescales. Subseasonally, precipitation and soil moisture explain nearly all the terrestrial water budget variability in the southern basins, while the northern latitudes are snow‐dominated regimes. Seasonal assessments reveal greater differences among the basins. Precipitation, evaporation, and runoff are the dominant sources of variability at lower latitudes, while at higher latitudes, terrestrial water storage in the form of ground snowpack and soil moisture has the leading role. Differences in land cover categorizations, for example, croplands, forests, or urban zones, further induce spatial differences in the hydrological characteristics. This quantification of variability in the terrestrial water cycle embedded at different temporal scales is important to assess the impacts of changes in climate and land cover on catchment sensitivities across the diverse hydroclimate of the Great Lakes region.

 

We use TROPOMI (TROPOspheric Monitoring Instrument) tropospheric nitrogen dioxide (NO₂) measurements to identify cropland soil nitrogen oxide (NO_x = NO + NO₂) emissions at daily to seasonal scales in the U.S. Southern Mississippi River Valley. Evaluating 1.5 years of TROPOMI observations with a box model, we observe seasonality in local NO_xenhancements and estimate maximum cropland soil NO_xemissions (15–34 ng N m⁻² s⁻¹) early in growing season (May–June). We observe soil NO_xpulsing in response to daily decreases in volumetric soil moisture (VSM) as measured by the Soil Moisture Active Passive (SMAP) satellite. Daily NO₂enhancements reach up to 0.8 × 10¹⁵ molecules cm⁻²4–8 days after precipitation when VSM decreases to ~30%, reflecting emissions behavior distinct from previously defined soil NO_xpulse events. This demonstrates that TROPOMI NO₂observations, combined with observations of underlying process controls (e.g., soil moisture), can constrain soil NO_xprocesses from space.

 

ABSTRACT To explore the various couplings across space and time and between ecosystems in a consistent manner, atmospheric modeling is moving away from the fractured limited-scale modeling strategy of the past toward a unification of the range of scales inherent in the Earth system. This paper describes the forward-looking Multi-Scale Infrastructure for Chemistry and Aerosols (MUSICA), which is intended to become the next-generation community infrastructure for research involving atmospheric chemistry and aerosols. MUSICA will be developed collaboratively by the National Center for Atmospheric Research (NCAR) and university and government researchers, with the goal of serving the international research and applications communities. The capability of unifying various spatiotemporal scales, coupling to other Earth system components, and process-level modularization will allow advances in both fundamental and applied research in atmospheric composition, air quality, and climate and is also envisioned to become a platform that addresses the needs of policy makers and stakeholders. 

Clouds can modify terrestrial productivity by reducing total surface radiation and increasing diffuse radiation, which may be more evenly distributed through plant canopies and increase ecosystem carbon uptake (the “diffuse fertilization effect”). Previous work at ecosystem-level observational towers demonstrated that diffuse photosynthetically active radiation (PAR; 400–700 nm) increases with cloud optical thickness (COT) until a COT of approximately 10, defined here as the “low-COT regime.” To identify whether the low-COT regime also influences carbon uptake on broader spatial and longer temporal time scales, we use global, monthly data to investigate the influence of COT on carbon uptake in three land-cover types: shrublands, forests, and croplands. While there are limitations in global gross primary production (GPP) products, global COT data derived from Moderate Resolution Imaging Spectroradiometer (MODIS) reveal that during the growing season tropical and subtropical regions more frequently experience a monthly low-COT regime (>20% of the time) than other regions of the globe. Contrary to ecosystem-level studies, comparisons of monthly COT with monthly satellite-derived solar-induced chlorophyll fluorescence and modeled GPP indicate that, although carbon uptake generally increases with COT under the low-COT regime, the correlations between COT and carbon uptake are insignificant (p > 0.05) in shrublands, forests, and croplands at regional scales. When scaled globally, vegetated regions under the low-COT regime account for only 4.9% of global mean annual GPP, suggesting that clouds and their diffuse fertilization effect become less significant drivers of terrestrial carbon uptake at broader spatial and temporal scales.