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We present a multiline survey of the interstellar medium (ISM) in two z > 6 quasar host galaxies, PJ231−20 ( z = 6.59) and PJ308−21 ( z = 6.23), and their two companion galaxies. Observations were carried out using the Atacama Large (sub-)Millimeter Array (ALMA). We targeted 11 transitions including atomic fine-structure lines (FSLs) and molecular lines: [NII] 205 μm , [CI] 369 μm , CO ( J up = 7, 10, 15, 16), H 2 O 3 12 − 2 21 , 3 21 − 3 12 , 3 03 − 2 12 , and the OH 163 μm doublet. The underlying far-infrared (FIR) continuum samples the Rayleigh-Jeans tail of the respectivemore »Free, publicly-accessible full text available August 1, 2022