We present nuclear magnetic resonance data in BaFe2As2 in the presence of pulsed strain fields that are interleaved in time with the radio frequency excitation pulses. In this approach, the preceding nuclear magnetization acquires a phase shift that is proportional to the strain and pulse time. The sensitivity of this approach is limited by the homogeneous decoherence time, T2, rather than the inhomogeneous linewidth. We measure the nematic susceptibility as a function of temperature and demonstrate a three orders of magnitude improvement in sensitivity. This approach will enable studies of the strain response in a broad range of materials that previously were inaccessible due to inhomogeneous broadening.
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Nuclear magnetic resonance provides a wealth of information about the magnetic and nematic degrees of freedom in the iron-based superconductors. A striking observation is that the spin lattice relaxation rate is inhomogeneous with a standard deviation that correlates with the nematic susceptibility. Moreover, the spin lattice relaxation is strongly affected by uniaxial strain, and in doped samples it depends sensitively upon the history of the applied strain. These observations suggest that quenched strain fields associated with doping atoms induce a nematic glass in the iron pnictide materials.more » « less
