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Free, publicly-accessible full text available March 1, 2026
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Taghinejad, Mohammad; Xia, Chenyi; Hrton, Martin; Lee, Kyu-Tae; Kim, Andrew S; Li, Qitong; Guzelturk, Burak; Kalousek, Radek; Xu, Fenghao; Cai, Wenshan; et al (, Science)Understanding the ultrafast excitation and transport dynamics of plasmon-driven hot carriers is critical to the development of optoelectronics, photochemistry, and solar-energy harvesting. However, the ultrashort time and length scales associated with the behavior of these highly out-of-equilibrium carriers have impaired experimental verification of ab initio quantum theories. Here, we present an approach to studying plasmonic hot-carrier dynamics that analyzes the temporal waveform of coherent terahertz bursts radiated by photo-ejected hot carriers from designer nano-antennas with a broken symmetry. For ballistic carriers ejected from gold antennas, we find an ~11-femtosecond timescale composed of the plasmon lifetime and ballistic transport time. Polarization- and phase-sensitive detection of terahertz fields further grant direct access to their ballistic transport trajectory. Our approach opens explorations of ultrafast carrier dynamics in optically excited nanostructures.more » « less
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Sie, Edbert J; Othman, Mohamed_A K; Nyby, Clara M; Pemmaraju, Das; Garcia, Christina_A C; Wang, Yaxian; Guzelturk, Burak; Xia, Chenyi; Xiao, Jun; Poletayev, Andrey; et al (, Nano Letters)
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