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Semiconductor moiré superlattices, characterized by their periodic spatial light emission, unveil a new paradigm of engineered photonic materials. Here, we show that ferroelectric moiré domains formed in a twisted hexagonal boron nitride (t-hBN) substrate can modulate light emission from an adjacent semiconductor MoSe2monolayer. The electrostatic potential at the surface of the t-hBN substrate provides a simple way to confine excitons in the MoSe2monolayer. The excitons confined within the domains and at the domain walls are spectrally separated because of a pronounced Stark shift. Moreover, the patterned light emission can be dynamically controlled by electrically gating the ferroelectric domains, introducing a functionality beyond other semiconductor moiré superlattices. Our findings chart an exciting pathway for integrating nanometer-scale moiré ferroelectric domains with various optically active functional layers, paving the way for advanced nanophotonics and metasurfaces.more » « lessFree, publicly-accessible full text available May 9, 2026
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Zhu, Jiayi; Zheng, Huiyuan; Wang, Xi; Park, Heonjoon; Xiao, Chengxin; Zhang, Yinong; Taniguchi, Takashi; Watanabe, Kenji; Yan, Jiaqiang; Gamelin, Daniel_R; et al (, Physical Review Letters)
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Zhang, Yinong; Xiao, Chengxin; Ovchinnikov, Dmitry; Zhu, Jiayi; Wang, Xi; Taniguchi, Takashi; Watanabe, Kenji; Yan, Jiaqiang; Yao, Wang; Xu, Xiaodong (, Nature Nanotechnology)
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Wang, Xi; Xiao, Chengxin; Park, Heonjoon; Zhu, Jiayi; Wang, Chong; Taniguchi, Takashi; Watanabe, Kenji; Yan, Jiaqiang; Xiao, Di; Gamelin, Daniel R.; et al (, Nature)
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