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This paper reports the development and detailed properties of about 13 metric tons of gadolinium sulfate octahydrate, $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$, which has been dissolved into Super-Kamiokande (SK) in the summer of 2020. We evaluate the impact of radioactive impurities in $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ on diffuse supernova neutrino background searches and solar neutrino observation and confirm the need to reduce radioactive and fluorescent impurities by about three orders of magnitude from commercially available high-purity $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$. In order to produce ultra-high-purity $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$, we have developed a method to remove impurities from gadolinium oxide, Gd2O3, consisting of acid dissolution, solvent extraction, and pH control processes, followed by a high-purity sulfation process. All of the produced ultra-high-purity $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ is assayed by inductively coupled plasma mass spectrometry and high-purity germanium detectors to evaluate its quality. Because of the long measurement time of high-purity germanium detectors, we have employed several underground laboratories for making parallel measurements including the Laboratorio Subterráneo de Canfranc in Spain, Boulby in the UK, and Kamioka in Japan. In the first half of production, the measured batch purities were found to be consistent with themore »specifications. However, in the latter half, the $\rm Gd_2(\rm SO_4)_3\cdot \rm 8H_2O$ contained one order of magnitude more 228Ra than the budgeted mean contamination. This was correlated with the corresponding characteristics of the raw material Gd2O3, in which an intrinsically large contamination was present. Based on their modest impact on SK physics, they were nevertheless introduced into the detector. To reduce 228Ra for the next stage of gadolinium loading to SK, a new process has been successfully established.

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Abstract Three-body nuclear forces play an important role in the structure of nuclei and hypernuclei and are also incorporated in models to describe the dynamics of dense baryonic matter, such as in neutron stars. So far, only indirect measurements anchored to the binding energies of nuclei can be used to constrain the three-nucleon force, and if hyperons are considered, the scarce data on hypernuclei impose only weak constraints on the three-body forces. In this work, we present the first direct measurement of the p–p–p and p–p– $$\Lambda $$ Λ systems in terms of three-particle correlation functions carried out for pp collisions at $$\sqrt{s} = 13$$ s = 13 TeV. Three-particle cumulants are extracted from the correlation functions by applying the Kubo formalism, where the three-particle interaction contribution to these correlations can be isolated after subtracting the known two-body interaction terms. A negative cumulant is found for the p–p–p system, hinting to the presence of a residual three-body effect while for p–p– $$\Lambda $$ Λ the cumulant is consistent with zero. This measurement demonstrates the accessibility of three-baryon correlations at the LHC.

Abstract A newly developed observable for correlations between symmetry planes, which characterize the direction of the anisotropic emission of produced particles, is measured in Pb–Pb collisions at $$\sqrt{s_\text {NN}}$$ s NN  = 2.76 TeV with ALICE. This so-called Gaussian Estimator allows for the first time the study of these quantities without the influence of correlations between different flow amplitudes. The centrality dependence of various correlations between two, three and four symmetry planes is presented. The ordering of magnitude between these symmetry plane correlations is discussed and the results of the Gaussian Estimator are compared with measurements of previously used estimators. The results utilizing the new estimator lead to significantly smaller correlations than reported by studies using the Scalar Product method. Furthermore, the obtained symmetry plane correlations are compared to state-of-the-art hydrodynamic model calculations for the evolution of heavy-ion collisions. While the model predictions provide a qualitative description of the data, quantitative agreement is not always observed, particularly for correlators with significant non-linear response of the medium to initial state anisotropies of the collision system. As these results provide unique and independent information, their usage in future Bayesian analysis can further constrain our knowledge on the properties of the QCD matter produced inmore »ultrarelativistic heavy-ion collisions.« less

Abstract This article presents measurements of the groomed jet radius and momentum splitting fraction in pp collisions at $$ \sqrt{s} $$ s = 5 . 02 TeV with the ALICE detector at the Large Hadron Collider. Inclusive charged-particle jets are reconstructed at midrapidity using the anti- k T algorithm for transverse momentum $$ 60<{p}_{\textrm{T}}^{\textrm{ch}\;\textrm{jet}}<80 $$ 60 < p T ch jet < 80 GeV/ c . We report results using two different grooming algorithms: soft drop and, for the first time, dynamical grooming. For each grooming algorithm, a variety of grooming settings are used in order to explore the impact of collinear radiation on these jet substructure observables. These results are compared to perturbative calculations that include resummation of large logarithms at all orders in the strong coupling constant. We find good agreement of the theoretical predictions with the data for all grooming settings considered.