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Sreenivasan, S.V. (Ed.)A major challenge of the large-scale application of two-dimensional (2D) materials is the scaling up of the process for its growth and transfer. Mechanical peeling has been demonstrated to be a promising method for transferring graphene in a fast and environmentally friendly manner. However, efforts in scaling up the process have been lacking. Performing mechanical peeling using a roll-to-roll (R2R) system could significantly increase the throughput of graphene transfer. Such a R2R process does not exist in industry. In this paper a novel R2R mechanical peeling system that has both speed and tension control capabilities is presented. Controllers that controlmore »Free, publicly-accessible full text available December 17, 2022