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This paper details the first application of a software tagging algorithm to reduce radon-induced backgrounds in liquid noble element time projection chambers, such as XENON1T and XENONnT. The convection velocity field in XENON1T was mapped out using${}^{222}\mathrm{Rn}$and${}^{218}\mathrm{Po}$events, and the rms convection speed was measured to be$0.30\pm 0.01\mathrm{cm}/\mathrm{s}$. Given this velocity field,${}^{214}\mathrm{Pb}$background events can be tagged when they are followed by${}^{214}\mathrm{Bi}$and${}^{214}\mathrm{Po}$decays, or preceded by${}^{218}\mathrm{Po}$decays. This was achieved by evolving a point cloud in the direction of a measured convection velocity field, and searching for${}^{214}\mathrm{Bi}$and${}^{214}\mathrm{Po}$decays or${}^{218}\mathrm{Po}$decays within a volume defined by the point cloud. In XENON1T, this tagging system achieved a${}^{214}\mathrm{Pb}$background reduction of${6.2}_{-0.9}^{+0.4}\%$with an exposure loss of$1.8\pm 0.2\%$, despite the timescales of convection being smaller than the relevant decay times. We show that the performance can be improved in XENONnT, and that the performance of such a software-tagging approach can be expected to be further improved in a diffusion-limited scenario. Finally, a similar method might be useful to tag the cosmogenic${}^{137}\mathrm{Xe}$background, which is relevant to the search for neutrinoless double-beta decay.

Published by the American Physical Society2024 

In this work, we expand on the XENON1T nuclear recoil searches to study the individual signals of dark matter interactions from operators up to dimension eight in a chiral effective field theory (ChEFT) and a model of inelastic dark matter (iDM). We analyze data from two science runs of the XENON1T detector totaling$1\mathrm{t}\times \mathrm{yr}$exposure. For these analyses, we extended the region of interest from$[4.9,40.9]{\mathrm{keV}}_{\mathrm{NR}}$to$[4.9,54.4]{\mathrm{keV}}_{\mathrm{NR}}$to enhance our sensitivity for signals that peak at nonzero energies. We show that the data are consistent with the background-only hypothesis, with a small background overfluctuation observed peaking between 20 and$50{\mathrm{keV}}_{\mathrm{NR}}$, resulting in a maximum local discovery significance of$1.7\sigma$for the$\mathrm{Vector}\otimes {\text{Vector}}_{\text{strange}}$ChEFT channel for a dark matter particle of$70\mathrm{GeV}/c^2$and$1.8\sigma$for an iDM particle of$50\mathrm{GeV}/c^2$with a mass splitting of$100\mathrm{keV}/c^2$. For each model, we report 90% confidence level upper limits. We also report upper limits on three benchmark models of dark matter interaction using ChEFT where we investigate the effect of isospin-breaking interactions. We observe rate-driven cancellations in regions of the isospin-breaking couplings, leading to up to 6 orders of magnitude weaker upper limits with respect to the isospin-conserving case.

Published by the American Physical Society2024 

This chapter is intended to help make inroads to the role of Intralipid in photodynamic therapy (PDT). In addition to Intralipid’s favorable property as a light scattering agent, we hypothesized that it will be unstable to photosensitized oxidation. To explore this, measurements of total quenching rate constants (kT) of singlet oxygen with Intralipid and its constituents are described. Furthermore, organic phosphines were tested to trap Intralipid peroxides formed in photosensitized oxidation reactions. Our findings indicate that the vulnerability of Intralipid to photooxidation might suggest limits of its use in PDT.