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Angle-resolved photoemission spectroscopy (ARPES) is a powerful tool for probing the momentum-resolved single-particle spectral function of materials. Historically, in situ magnetic fields have been carefully avoided as they are detrimental to the control of photoelectron trajectory during the photoelectron detection process. However, magnetic field is an important experimental knob for both probing and tuning symmetry-breaking phases and electronic topology in quantum materials. In this paper, we introduce an easily implementable method for realizing an in situ tunable magnetic field at the sample position in an ARPES experiment and analyze magnetic-field-induced artifacts in the ARPES data. Specifically, we identified and quantified three distinct extrinsic effects of a magnetic field: constant energy contour rotation, emission angle contraction, and momentum broadening. We examined these effects in three prototypical quantum materials, i.e., a topological insulator (Bi2Se3), an iron-based superconductor (LiFeAs), and a cuprate superconductor (Pb-Bi2Sr2CuO6+x), and demonstrate the feasibility of ARPES measurements in the presence of a controllable magnetic field. Our studies lay the foundation for the future development of the technique and interpretation of ARPES measurements of field-tunable quantum phases. 

Terahertz (THz) magnetoresistance effects have been extensively investigated and have shown promising results for applications in magnetic modulations of the amplitude of THz waves. However, THz magnetocapacitance in dielectric systems, which is essential for phase modulations of THz radiation, remains largely unexplored. Here, we study the THz response of a bulk single crystal of La_0.875Sr_0.125MnO₃at around its Curie temperature, observing significant magnetic-field-induced changes in the THz resistance and capacitance extracted from the optical conductivity. We discuss possible mechanisms for the observed coexistence of colossal THz magnetoresistance and magnetocapacitance in a perovskite manganite that is not multiferroic. This work enhances our understanding of colossal magnetoresistance in a complex system with THz spectroscopy and demonstrates potential use of perovskite manganites in THz technology.

 

For easy manipulation of polarization states of light for applications in communications, imaging, and information processing, an efficient mechanism is desired for rotating light polarization with a minimum interaction length. Here, we report giant polarization rotations for terahertz (THz) electromagnetic waves in ultrathin ($\sim <\#comment/>45\mathrm{n}\mathrm{m}$), high-density films of aligned carbon nanotubes. We observed polarization rotations of up to$\sim <\#comment/>{20}^{\circ <\#comment/>}$and$\sim <\#comment/>{110}^{\circ <\#comment/>}$for transmitted and reflected THz pulses, respectively. The amount of polarization rotation was a sensitive function of the angle between the incident THz polarization and the nanotube alignment direction, exhibiting a “magic” angle at which the total rotation through transmission and reflection becomes exactly 90°. Our model quantitatively explains these giant rotations as a result of extremely anisotropic optical constants, demonstrating that aligned carbon nanotubes promise ultrathin, broadband, and tunable THz polarization devices.

 

Hybrid light–matter coupled states, or polaritons, in magnetic materials have attracted significant attention due to their potential for enabling novel applications in spintronics and quantum information processing. However, most magnon‐polariton studies in the strong coupling regime to date have been carried out for ferromagnetic materials with magnon excitations at gigahertz frequencies. Here, strong resonant photon–magnon coupling at frequencies above 1 terahertz is investigated for the first time in a prototypical room‐temperature antiferromagnetic insulator, NiO,  inside a Fabry–Pérot cavity. The cavity is formed by the crystal itself with a thickness adjusted to an optimal value. Terahertz time‐domain spectroscopy measurements in magnetic fields up to 25 T reveal the evolution of the magnon frequency through Fabry–Pérot cavity modes with photon–magnon anticrossing behavior, demonstrating clear vacuum Rabi splittings exceeding the polariton linewidths. These results show that NiO is a promising platform for exploring antiferromagnetic spintronics and cavity magnonics in the terahertz frequency range.

 

Carbon nanotubes (CNTs) possess extremely anisotropic electronic, thermal, and optical properties owing to their 1D character. While their linear optical properties have been extensively studied, nonlinear optical processes, such as harmonic generation for frequency conversion, remain largely unexplored in CNTs, particularly in macroscopic CNT assemblies. In this work, macroscopic films of aligned and type‐separated (semiconducting and metallic) CNTs are synthesized and polarization‐dependent third‐harmonic generation (THG) from the films with fundamental wavelengths ranging from 1.5 to 2.5 µm is studied. Both films exhibited strongly wavelength‐dependent, intense THG signals, enhanced through exciton resonances, and third‐order nonlinear optical susceptibilities of 2.50 × 10⁻¹⁹ m² V⁻²(semiconducting CNTs) and 1.23 × 10⁻¹⁹ m² V⁻²(metallic CNTs), respectively are found, for 1.8 µm excitation. Further, through systematic polarization‐dependent THG measurements, the values of all elements of the susceptibility tensor are determined, verifying the macroscopically 1D nature of the films. Finally, polarized THG imaging is performed to demonstrate the nonlinear anisotropy in the large‐size CNT film with good alignment. These findings promise applications of aligned CNT films in mid‐infrared frequency conversion, nonlinear optical switching, polarized pulsed lasers, polarized long‐wave detection, and high‐performance anisotropic nonlinear photonic devices.

 

In terahertz (THz) photonics, there is an ongoing effort to develop thin, compact devices such as dielectric photonic crystal (PhC) slabs with desirable light–matter interactions. However, previous works in THz PhC slabs have been limited to rigid substrates with thicknesses$\sim <\#comment/>100\mathrm{s}$of micrometers. Dielectric PhC slabs have been shown to possess in-plane modes that are excited by external radiation to produce sharp guided-mode resonances with minimal absorption for applications in sensors, optics, and lasers. Here we confirm the existence of guided resonances in a membrane-type THz PhC slab with subwavelength (${\mathrm{\lambda <\#comment/>}}_0/6-<\#comment/>{\mathrm{\lambda <\#comment/>}}_0/12$) thicknesses of flexible dielectric polyimide films. The transmittance of the guided resonances was measured for different structural parameters of the unit cell. Furthermore, we exploited the flexibility of the samples to modulate the guided modes for a bend angle of$\mathrm{\theta <\#comment/>}\ge <\#comment/>5^{\circ <\#comment/>}$, confirmed experimentally by the suppression of these modes. The mechanical flexibility of the device allows for an additional degree of freedom in system design for high-speed communications, soft wearable photonics, and implantable medical devices.

 

Hybrid material systems are a promising approach for extending the capabilities of silicon photonics. Given the weak electro‐optic and thermo‐optic effects in silicon, there is intense interest in integrating an ultrafast‐switching phase‐change material with a large refractive index contrast into the waveguide, such as vanadium dioxide (VO₂). It is well established that the phase transition in VO₂thin films can be triggered by ultrafast, 800 nm laser pulses, and that pump‐laser fluence is a critical determinant of the recovery time of thin films irradiated by femtosecond pulses. However, thin‐film experiments are not reliable guides to a VO₂:Si system for all‐optical, on‐chip switching because of the differences in VO₂optical constants in the telecommunication band, and the complex sample geometry and alignment issues in a waveguide geometry. This paper reports the first demonstration that the reversible, ultrafast photoinduced phase transition in VO₂can achieve sub‐picosecond response when small VO₂volumes are integrated into a silicon waveguide as the active element. The result suggests that VO₂can be pursued as a strong candidate for waveguide switching with sub‐picosecond on‐off times.