Many technologically useful magnetic oxides are ferrimagnetic insulators, which consist of chemically distinct cations. Here, we examine the spin dynamics of different magnetic cations in ferrimagnetic NiZnAl-ferrite (Ni0.65Zn0.35Al0.8Fe1.2O4) under continuous microwave excitation. Specifically, we employ time-resolved x-ray ferromagnetic resonance to separately probe Fe2+/3+ and Ni2+ cations on different sublattice sites. Our results show that the precessing cation moments retain a rigid, collinear configuration to within ≈2°. Moreover, the effective spin relaxation is identical to within <10% for all magnetic cations in the ferrite. Thus, we validate the oft-assumed “ferromagnetic-like” dynamics in the resonantly driven ferrimagnetic oxide: the magnetic moments from different cations precess as a coherent, collective magnetization, despite the high contents of nonmagnetic Zn2+ and Al3+ diluting the exchange interactions.
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Knut, R ; Malik, R S ; Kons, C ; Shoup, J E ; Radu, F ; Luo, C ; Kvashnin, Y O ; Gupta, A ; Karis, O ; Arena, D A ( , Journal of Physics: Condensed Matter)Abstract Strained materials can exhibit drastically modified physical properties in comparison to their fully relaxed analogues. We report on the x-ray absorption spectra (XAS) and magnetic circular dichroism (XMCD) of a strained NiFe 2 O 4 inverse spinel film grown on a symmetry matched single crystal MgGa 2 O 4 substrate. The Ni XAS spectra exhibit a sizable difference in the white line intensity for measurements with the x-ray electric field parallel to the film plane (normal incidence) vs when the electric field is at an angle (off-normal). A considerable difference is also observed in the Fe L 2,3 XMCD spectrum. Modeling of the XAS and XMCD spectra indicate that the modified energy ordering of the cation 3 d states in the strained film leads to a preferential filling of 3 d states with out-of-plane character. In addition, the results point to the utility of x-ray spectroscopy in identifying orbital populations even with elliptically polarized x-rays.more » « less
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Liu, H. ; Knut, R. ; Saha, S. ; Malik, R. S. ; Jatkar, K. ; Stefanuik, R. ; Söderström, J. ; Shoup, J. E. ; Khadka, Durga ; Thapaliya, T. R. ; et al ( , Journal of Applied Physics)