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Creators/Authors contains: "Kwon, Minho"

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  1. Free, publicly-accessible full text available May 1, 2024
  2. We report on the design and characterization of a cold atom source for strontium (Sr) based on a two-dimensional magneto-optical trap (MOT) that is directly loaded from the atom jet of a dispenser. We characterize the atom flux of the source by measuring the loading rate of a three-dimensional MOT. We find loading rates of up to 10 8 atoms per second. The setup is compact, easy to construct, and has low power consumption. It addresses the longstanding challenge of reducing the complexity of cold beam sources for Sr, which is relevant for optical atomic clocks, quantum simulation, and computing devices based on ultracold Sr. 
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  3. We propose metasurface holograms as a novel platform to generate optical trap arrays for cold atoms with high fidelity, efficiency, and thermal stability. We developed design and fabrication methodologies to create dielectric, phase-only metasurface holograms based on titanium dioxide. We experimentally demonstrated optical trap arrays of various geometries, including periodic and aperiodic configurations with dimensions ranging from 1D to 3D and the number of trap sites up to a few hundred. We characterized the performance of the holographic metasurfaces in terms of the positioning accuracy, size and intensity uniformity of the generated traps, and power handling capability of the dielectric metasurfaces. Our proposed platform has great potential for enabling fundamental studies of quantum many-body physics, and quantum simulation and computation tasks. The compact form factor, passive nature, good power handling capability, and scalability of generating high-quality, large-scale arrays also make the metasurface platform uniquely suitable for realizing field-deployable devices and systems based on cold atoms. 
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  5. We present a continuous, narrow-linewidth, tunable laser system that outputs up to 14.0 W at 770 nm. The light is generated by frequency doubling 18.8 W of light from a 1540 nm fiber amplifier that is seeded by a single-mode diode laser achieving><#comment/>74%<#comment/>conversion efficiency. We utilize a lithium triborate crystal in an enhancement ring cavity. The low intensity noise and narrow linewidth of the 770 nm output are suitable for cold atom experiments.

     
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  6. Ensemble qubits with strong coupling to photons and resilience against single atom loss are promising candidates for building quantum networks. We report on progress towards high fidelity preparation and control of ensemble qubits using Rydberg blockade. Our previous demonstration of ensemble qubit preparation at a fidelity <60% was possibly limited by Rydberg blockade leakage due to uncontrolled short range atom pair separation. We show progress towards ensembles with a blue-detuned 1-D lattice on top of the existing red-detuned dipole trap, which will suppress unwanted Rydberg interactions by imposing constraints on the atomic separation. We study the effect of lattice insertion on the fidelity of ensemble state preparation and Rydberg-mediated gates. Studies of cooperative scattering from a 1D atomic array will also be presented. 
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  7. Abstract

    The production of elemental sulfur from petroleum refining has created a technological opportunity to increase the valorization of elemental sulfur by the creation of high‐performance sulfur based plastics with improved thermomechanical properties, elasticity and flame retardancy. We report on a synthetic polymerization methodology to prepare the first example of sulfur based segmented multi‐block polyurethanes (SPUs) and thermoplastic elastomers that incorporate an appreciable amount of sulfur into the final target material. This approach applied both the inverse vulcanization of S8with olefinic alcohols and dynamic covalent polymerizations with dienes to prepare sulfur polyols and terpolyols that were used in polymerizations with aromatic diisocyanates and short chain diols. Using these methods, a new class of high molecular weight, soluble block copolymer polyurethanes were prepared as confirmed by Size Exclusion Chromatography, NMR spectroscopy, thermal analysis, and microscopic imaging. These sulfur‐based polyurethanes were readily solution processed into large area free standing films where both the tensile strength and elasticity of these materials were controlled by variation of the sulfur polyol composition. SPUs with both high tensile strength (13–24 MPa) and ductility (348 % strain at break) were prepared, along with SPU thermoplastic elastomers (578 % strain at break) which are comparable values to classical thermoplastic polyurethanes (TPUs). The incorporation of sulfur into these polyurethanes enhanced flame retardancy in comparison to classical TPUs, which points to the opportunity to impart new properties to polymeric materials as a consequence of using elemental sulfur.

     
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  8. Abstract

    The production of elemental sulfur from petroleum refining has created a technological opportunity to increase the valorization of elemental sulfur by the creation of high‐performance sulfur based plastics with improved thermomechanical properties, elasticity and flame retardancy. We report on a synthetic polymerization methodology to prepare the first example of sulfur based segmented multi‐block polyurethanes (SPUs) and thermoplastic elastomers that incorporate an appreciable amount of sulfur into the final target material. This approach applied both the inverse vulcanization of S8with olefinic alcohols and dynamic covalent polymerizations with dienes to prepare sulfur polyols and terpolyols that were used in polymerizations with aromatic diisocyanates and short chain diols. Using these methods, a new class of high molecular weight, soluble block copolymer polyurethanes were prepared as confirmed by Size Exclusion Chromatography, NMR spectroscopy, thermal analysis, and microscopic imaging. These sulfur‐based polyurethanes were readily solution processed into large area free standing films where both the tensile strength and elasticity of these materials were controlled by variation of the sulfur polyol composition. SPUs with both high tensile strength (13–24 MPa) and ductility (348 % strain at break) were prepared, along with SPU thermoplastic elastomers (578 % strain at break) which are comparable values to classical thermoplastic polyurethanes (TPUs). The incorporation of sulfur into these polyurethanes enhanced flame retardancy in comparison to classical TPUs, which points to the opportunity to impart new properties to polymeric materials as a consequence of using elemental sulfur.

     
    more » « less