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Five new near-infrared (NIR) phosphorescent bis-cyclometalated iridium( iii ) complexes, partnering highly conjugated cyclometalating ligands with quinoline-derived ancillary ligands, have been developed. These complexes have peak NIR luminescence wavelengths from 711 to 729 nm, with photoluminescence quantum yields ranging from 0.042 to 0.36.more » « less
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Lee, Kyounghoon ; Lai, Po-Ni ; Parveen, Riffat ; Donahue, Courtney M. ; Wymore, Mikayla M. ; Massman, Blake A. ; Vlaisavljevich, Bess ; Teets, Thomas S. ; Daly, Scott R. ( , Chemical Communications)Here we report how reactions at a chemically reactive diphosphine shift the long-lived luminescent colour of a crystalline three-coordinate Cu( i ) complex from green to blue. The results demonstrate how vapochromism and single-crystal-to-single-crystal transformations can be achieved using ligand-centered reactions.more » « less
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Lai, Po−Ni ; Yoon, Sungwon ; Wu, Yumeng ; Teets, Thomas S. ( , ACS Organic & Inorganic Au)
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Liska, Tadeas ; Swetz, Anna ; Lai, Po‐Ni ; Zeller, Matthias ; Teets, Thomas S. ; Gray, Thomas G. ( , Chemistry – A European Journal)
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Li, Zhong'an ; Toivola, Ryan ; Ding, Feizhi ; Yang, Jeffrey ; Lai, Po‐Ni ; Howie, Tucker ; Georgeson, Gary ; Jang, Sei‐Hum ; Li, Xiaosong ; Flinn, Brian D. ; et al ( , Advanced Materials)