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Creators/Authors contains: "Schnell, Jordan L."

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  1. Abstract

    Electric vehicles (EVs) constitute just a fraction of the current U.S. transportation fleet; however, EV market share is surging. EV adoption reduces on-road transportation greenhouse gas emissions by decoupling transportation services from petroleum, but impacts on air quality and public health depend on the nature and location of vehicle usage and electricity generation. Here, we use a regulatory-grade chemical transport model and a vehicle-to-electricity generation unit electricity assignment algorithm to characterize neighborhood-scale (∼1 km) air quality and public health benefits and tradeoffs associated with a multi-modal EV transition. We focus on a Chicago-centric regional domain wherein 30% of the on-road transportation fleet is instantaneously electrified and changes in on-road, refueling, and power plant emissions are considered. We find decreases in annual population-weighted domain mean NO2(−11.83%) and PM2.5(−2.46%) with concentration reductions of up to −5.1 ppb and −0.98µg m−3in urban cores. Conversely, annual population-weighted domain mean maximum daily 8 h average ozone (MDA8O3) concentrations increase +0.64%, with notable intra-urban changes of up to +2.3 ppb. Despite mixed pollutant concentration outcomes, we find overall positive public health outcomes, largely driven by NO2concentration reductions that result in outsized mortality rate reductions for people of color, particularly for the Black populations within our domain.

     
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  2. Wildfires and meteorological conditions influence the co-occurrence of multiple harmful air pollutants including fine particulate matter (PM 2.5 ) and ground-level ozone. We examine the spatiotemporal characteristics of PM 2.5 /ozone co-occurrences and associated population exposure in the western United States (US). The frequency, spatial extent, and temporal persistence of extreme PM 2.5 /ozone co-occurrences have increased significantly between 2001 and 2020, increasing annual population exposure to multiple harmful air pollutants by ~25 million person-days/year. Using a clustering methodology to characterize daily weather patterns, we identify significant increases in atmospheric ridging patterns conducive to widespread PM 2.5 /ozone co-occurrences and population exposure. We further link the spatial extent of co-occurrence to the extent of extreme heat and wildfires. Our results suggest an increasing potential for co-occurring air pollution episodes in the western US with continued climate change. 
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  3. Abstract

    The southern Lake Michigan region of the United States, home to Chicago, Milwaukee, and other densely populated Midwestern cities, frequently experiences high pollutant episodes with unevenly distributed exposure and health burdens. Using the two‐way coupled Weather Research Forecast and Community Multiscale Air Quality Model (WRF‐CMAQ), we investigate criteria pollutants over a southern Lake Michigan domain using 1.3 and 4 km resolution hindcast simulations. We assess WRF‐CMAQ's performance using data from the National Climatic Data Center and Environmental Protection Agency Air Quality System. Our 1.3 km simulation slightly improves on the 4 km simulation's meteorological and chemical performance while also resolving key details in areas of high exposure and impact, that is, urban environments. At 1.3 km, we find that most air quality‐relevant meteorological components of WRF‐CMAQ perform at or above community benchmarks. WRF‐CMAQ's chemical performance also largely meets community standards, with substantial nuance depending on the performance metric and component assessed. For example, hourly simulated NO2and O3are highly correlated with observations (r > 0.6) while PM2.5is less so (r = 0.4). Similarly, hourly simulated NO2and PM2.5have low biases (<10%), whereas O3biases are larger (>30%). Simulated spatial pollutant patterns show distinct urban‐rural footprints, with urban NO2and PM2.520%–60% higher than rural, and urban O36% lower. We use our 1.3 km simulations to resolve high‐pollution areas within individual urban neighborhoods and characterize seasonal changes in O3regimes across tight spatial gradients. Our findings demonstrate both the benefits and limitations of high‐resolution simulations, particularly over urban settings.

     
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  4. Abstract

    Storylines of atmospheric circulation change, or physically self-consistent narratives of plausible future events, have recently been proposed as a non-probabilistic means to represent uncertainties in climate change projections. Here, we apply the storyline approach to 21st century projections of summer air stagnation over Europe and the United States. We use a Climate Model Intercomparison Project Phase 6 (CMIP6) ensemble to generate stagnation storylines based on the forced response of three remote drivers of the Northern Hemisphere mid-latitude atmospheric circulation: North Atlantic warming, North Pacific warming, and tropical versus Arctic warming. Under a high radiative forcing scenario (SSP5-8.5), models consistently project increases in stagnation over Europe and the U.S., but the magnitude and spatial distribution of changes vary substantially across CMIP6 ensemble members, suggesting that future projections are not well-constrained when using the ensemble mean alone. We find that the diversity of projected stagnation changes depends on the forced response of remote drivers in individual models. This is especially true in Europe, where differences of ∼2 summer stagnant days per degree of global warming are found amongst the different storyline combinations. For example, the greatest projected increase in stagnation for most European regions leads to the smallest increase in stagnation for southwestern Europe; i.e. limited North Atlantic warming combined with near-equitable tropical and Arctic warming. In the U.S., only the atmosphere over the northern Rocky Mountain states demonstrates comparable stagnation projection uncertainty, due to opposite influences of remote drivers on the meteorological conditions that lead to stagnation.

     
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