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  1. ; ; ; ; ; ; ; (, Chemical Communications)
    Coordination of 1-isopropyl-3,5-dipyridyl-6-oxoverdazyl to cobalt results in a dication best described in the solid state as a high spin cobalt( ii ) ion coordinated to two radical ligands with an S = 3/2 ground state. On dissolution in acetonitrile, the cobalt( ii ) form equilibrates with a cobalt( iii ) valence tautomer with an S = 1/2 ground state. 
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