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Luo, Jiaming; Li, Shuyi; Ye, Zhipeng; Xu, Rui; Yan, Han; Zhang, Junjie; Ye, Gaihua; Chen, Lebing; Hu, Ding; Teng, Xiaokun; et al (, Nano Letters)
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Yang, Bowen; Goh, Yin Min; Sung, Suk Hyun; Ye, Gaihua; Biswas, Sananda; Kaib, David A.; Dhakal, Ramesh; Yan, Shaohua; Li, Chenghe; Jiang, Shengwei; et al (, Nature Materials)
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Lujan, David; Choe, Jeongheon; Rodriguez-Vega, Martin; Ye, Zhipeng; Leonardo, Aritz; Nunley, T. Nathan; Chang, Liang-Juan; Lee, Shang-Fan; Yan, Jiaqiang; Fiete, Gregory A.; et al (, Nature Communications)Abstract Electron band topology is combined with intrinsic magnetic orders in MnBi 2 Te 4 , leading to novel quantum phases. Here we investigate collective spin excitations (i.e. magnons) and spin fluctuations in atomically thin MnBi 2 Te 4 flakes using Raman spectroscopy. In a two-septuple layer with non-trivial topology, magnon characteristics evolve as an external magnetic field tunes the ground state through three ordered phases: antiferromagnet, canted antiferromagnet, and ferromagnet. The Raman selection rules are determined by both the crystal symmetry and magnetic order while the magnon energy is determined by different interaction terms. Using non-interacting spin-wave theory, we extract the spin-wave gap at zero magnetic field, an anisotropy energy, and interlayer exchange in bilayers. We also find magnetic fluctuations increase with reduced thickness, which may contribute to a less robust magnetic order in single layers.more » « less
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