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  1. Composites printed using material extrusion additive manufacturing (AM) typically exhibit alignment of high- aspect-ratio reinforcements parallel to the print direction. This alignment leads to highly anisotropic stiffness, strength, and transport properties. In many cases, it would be desirable to increase mechanical and transport properties transverse to the print direction, for example, in 3D-printed heat sinks or heat exchangers where heat must be moved efficiently between printed roads or layers. Rotational direct ink writing (RDIW), where the deposition nozzle simultaneously rotates and translates during deposition, provides a method to reorient fibers transverse to the print direction during the printing process. In the present work, carbon fiber-reinforced epoxy composites were printed by RDIW with a range of nozzle rotation rates and the in-plane and through-thickness thermal conductivity was measured. In addition, the orientation of carbon fiber (CF) in the composites was measured using optical microscopy and image analysis, from which second-order fiber orientation tensors were calculated. These results showed that the orientation of CF became less anisotropic as nozzle rotation rate increased, leading to increased through-thickness thermal conductivity, which increased by 40% at the highest rotation rate. The orientation tensors also showed that RDIW was more effective at reorienting fibers within the in-plane transverse direction compared to the through-thickness transverse direction. The results presented here demonstrate that a current weakness of material extrusion AM composites—poor thermal conductivity in the through-thickness direction—can be significantly improved with RDIW. 
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    Free, publicly-accessible full text available December 1, 2024
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    Purpose Mechanical anisotropy associated with material extrusion additive manufacturing (AM) complicates the design of complex structures. This study aims to focus on investigating the effects of design choices offered by material extrusion AM – namely, the choice of infill pattern – on the structural performance and optimality of a given optimized topology. Elucidation of these effects provides evidence that using design tools that incorporate anisotropic behavior is necessary for designing truly optimal structures for manufacturing via AM. Design/methodology/approach A benchmark topology optimization (TO) problem was solved for compliance minimization of a thick beam in three-point bending and the resulting geometry was printed using fused filament fabrication. The optimized geometry was printed using a variety of infill patterns and the strength, stiffness and failure behavior were analyzed and compared. The bending tests were accompanied by corresponding elastic finite element analyzes (FEA) in ABAQUS. The FEA used the material properties obtained during tensile and shear testing to define orthotropic composite plies and simulate individual printed layers in the physical specimens. Findings Experiments showed that stiffness varied by as much as 22% and failure load varied by as much as 426% between structures printed with different infill patterns. The observed failure modes were also highly dependent on infill patterns with failure propagating along with printed interfaces for all infill patterns that were consistent between layers. Elastic FEA using orthotropic composite plies was found to accurately predict the stiffness of printed structures, but a simple maximum stress failure criterion was not sufficient to predict strength. Despite this, FE stress contours proved beneficial in identifying the locations of failure in printed structures. Originality/value This study quantifies the effects of infill patterns in printed structures using a classic TO geometry. The results presented to establish a benchmark that can be used to guide the development of emerging manufacturing-oriented TO protocols that incorporate directionally-dependent, process-specific material properties. 
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