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Weakly, Robert B.; Gaynor, James D.; Khalil, Munira (, The Journal of Chemical Physics)
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Gaynor, James D.; Weakly, Robert B.; Khalil, Munira (, The Journal of Chemical Physics)
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Implementation of Broadband near-UV Pump Pulses for Ultrafast 2D Electronic-Vibrational SpectroscopySandwisch, Jason W.; Gaynor, James D.; Khalil, Munira (, Optica Publishing Group)We present the generation of efficient, tunable sub-20 fs broadband near UV pulses. The tunable pulses are used in two-dimensional electronic-vibrational spectroscopy and reveal additional vibronic states in an excited state intramolecular proton transfer process.more » « less
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Weakly, Robert B.; Gaynor, James D.; Khalil, Munira (, Optica Publishing Group)A model vibronic Hamiltonian composed of coupled anharmonic vibrational modes and two electronic states provides a quantitative framework for understanding how vibronic couplings and dipole orientations are encoded in two-dimensional vibronic spectroscopy.more » « less
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