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  1. We present the generation of efficient, tunable sub-20 fs broadband near UV pulses. The tunable pulses are used in two-dimensional electronic-vibrational spectroscopy and reveal additional vibronic states in an excited state intramolecular proton transfer process. 
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  2. A model vibronic Hamiltonian composed of coupled anharmonic vibrational modes and two electronic states provides a quantitative framework for understanding how vibronic couplings and dipole orientations are encoded in two-dimensional vibronic spectroscopy. 
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