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Lacy, John H; Patenotte, Gabriel E; Kinney, Abby C; Majumder, Protik K (, Photonics)We present a low-noise (<10 µrad/Hz) broadband Faraday Rotation Spectroscopy method which is feasible for near-ultraviolet through near-infrared wavelengths. We demonstrate this in the context of a high-precision spectroscopy experiment using a heated Pb vapor cell and two different lasers, one in the UV (368 nm) and a second in the IR (1279 nm). A key element of the experimental technique is the use of a uniaxial single crystal CeF3 Faraday modulator with excellent transmission and optical rotation properties across the aforementioned wavelength range. Polarimeter performance is assessed as a function of crystal orientation and alignment, AC modulation amplitude, laser power, and laser wavelength. Crystal-induced distortion of the (6p2)3P0→(6p2)3P1 (1279 nm) and (6p2)3P1→(6p7s)3P0 (368 nm) spectral lines due to misalignment-induced birefringence is discussed and modeled using the Jones calculus.more » « less
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Maser, Daniel L.; Hoenig, Eli; Wang, B.-Y.; Rupasinghe, P. M.; Porsev, S. G.; Safronova, M. S.; Majumder, P. K. (, Physical Review A)