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Characterization of Water Structure and Phase Behavior within Metal–Organic Nanotubes

https://doi.org/10.1021/acs.langmuir.3c02786

Jahinge, Tiron H. L. ; Payne, Maurice K. ; Unruh, Daniel K. ; Jayasinghe, Ashini S. ; Yu, Ping ; Forbes, Tori Z. ( December 2023 , Langmuir)
Impacts of Surface Adsorption on Water Uptake within a Metal Organic Nanotube Material

https://doi.org/10.1021/acs.langmuir.2c01124

Applegate, Lindsey C. ; Samarasiri, Vidumini S. ; Leddy, Johna ; Forbes, Tori Z. ( November 2022 , Langmuir)
Selectivity for water isotopologues within metal organic nanotubes

https://doi.org/10.1039/d1ra00602a

Payne, Maurice K. ; Applegate, Lindsey C. ; Singh, Priyanka ; Jayasinghe, Ashini S. ; Crull, George B. ; Grafton, Andrea B. ; Cheatum, Christopher M. ; Forbes, Tori Z. ( May 2021 , RSC Advances)
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Through a combination of many analytical approaches, we show that a metal organic nanotube (UMON) displays selectivity for H 2 O over all types of heavy water (D 2 O, HDO, HTO). Water adsorption experiments combined with vibrational and radiochemical analyses reveal significant differences in uptake and suggest that surface adsorption processes may be a key driver in water uptake for this material.
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