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We begin with a treatment of the Caputo time‐fractional diffusion equation, by using the Laplace transform, to obtain a Volterra integro‐differential equation. We derive and utilize a numerical scheme that is derived in parallel to the L1‐method for the time variable and a standard fourth‐order approximation in the spatial variable. The main method derived in this article has a rate of convergence ofO(k^α + h⁴)foru(x,t) ∈ C^α([0,T];C⁶(Ω)),0 < α < 1, which improves previous regularity assumptions that requireC²[0,T]regularity in the time variable. We also present a novel alternative method for a first‐order approximation in time, under a regularity assumption ofu(x,t) ∈ C¹([0,T];C⁶(Ω)), while exhibiting order of convergence slightly more thanO(k)in time. This allows for a much wider class of functions to be analyzed which was previously not possible under the L1‐method. We present numerical examples demonstrating these results and discuss future improvements and implications by using these techniques.