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A selenophene-containing conjugated organic ligand, 2-(4′-methyl-5′-(5-(3-methylthiophen-2-yl)selenophen-2-yl)-[2,2′-bithiophen]-5-yl)ethan-1-aminium (STm), was synthesized and incorporated into a Sn( ii )-based two-dimensional perovskite, (STm) 2 SnI 4 . The band offset between the perovskite and ligand can be fine-tuned by introducing the STm ligand. Both field-effect transistor and light-emitting diode devices based on (STm) 2 SnI 4 films exhibit high performance and enhanced operational stability.more » « less
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Liang, Aihui ; Gao, Yao ; Asadpour, Reza ; Wei, Zitang ; Finkenauer, Blake P. ; Jin, Linrui ; Yang, Jiaqi ; Wang, Kang ; Chen, Ke ; Liao, Peilin ; et al ( , Journal of the American Chemical Society)