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Gupta, Mayanak K.; Ding, Jingxuan; Osti, Naresh C.; Abernathy, Douglas L.; Arnold, William; Wang, Hui; Hood, Zachary; Delaire, Olivier (, Energy & Environmental Science)Strongly anharmonic low-energy phonons enable the fast diffusion of Na ions in the solid-state electrolyte compound Na3PS4.more » « less
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Halacoglu, Selim; Chertmanova, Sabina; Chen, Yan; Li, Yang; Rajapakse, Manthila; Sumanasekera, Gamini; Narayanan, Badri; Wang, Hui (, ChemSusChem)The structural evolutions and phase changes of Na3SbS4 and Na3SbS3.5Se0.5 conductor are revealed by in-situ neutron diffraction during their solid-state synthesis, sintering, and cooling process. The Na3SbS4 phase forms directly from precursors through a rapid solid reaction around 300 °C and changes to a molten state beyond 590 °C. Se doping affects the solid reaction temperatures, unit cell size, and structural stability.more » « less
