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Deformation experiments on hematite characterize its slip‐rate dependent frictional properties and deformation mechanisms. These data inform interpretations of slip behavior from exhumed hematite‐coated faults and present‐day deformation at depth. We used a rotary‐shear apparatus to conduct single‐velocity and velocity‐step experiments on polycrystalline specular hematite rock (∼17 μm average plate thickness) at slip rates of 0.85 μm/s to 320 mm/s, displacements of primarily 1–3 cm and up to 45 cm, and normal stresses of 5 and 8.5 MPa. The average coefficient of friction is 0.70; velocity‐step experiments indicate velocity‐strengthening to velocity‐neutral behavior at rates <1 mm/s. Scanning electron microscopy showed experimentally generated faults develop in a semi‐continuous, thin layer of red hematite gouge. Angular gouge particles have an average diameter of ∼0.7 μm, and grain size reduction during slip yields a factor of 10–100 increase in surface area. Hematite is amenable to (U‐Th)/He thermochronometry, which can quantify fault‐related thermal and mechanical processes. Comparison of hematite (U‐Th)/He dates from the undeformed material and experimentally produced gouge indicates He loss occurs during comminution at slow deformation rates without an associated temperature rise required for diffusive loss. Our results imply that, in natural fault rocks, deformation localizes within coarse‐grained hematite by stable sliding, and that hematite (U‐Th)/He dates acquired from ultracataclasite or highly comminuted gouge reflect minor He loss unrelated to thermal processes. Consequently, the magnitude of temperature rise and associated thermal resetting in hematite‐bearing fault rocks based on (U‐Th)/He thermochronometry may be overestimated if only diffusive loss of He is considered. 

Abstract Slow slip is part of the earthquake cycle, but the processes controlling this phenomenon in space and time are poorly constrained. Hematite, common in continental fault zones, exhibits unique textures and (U-Th)/He thermochronometry data patterns reflecting different slip rates. We investigated networks of small hematite-coated slip surfaces in basement fault damage of exhumed strike-slip faults that connect to the southern San Andreas fault in a flower structure in the Mecca Hills, California, USA. Scanning electron microscopy shows these millimeter-thick surfaces exhibit basal hematite injection veins and layered veinlets comprising nanoscale, high-aspect-ratio hematite plates akin to phyllosilicates. Combined microstructural and hematite (U-Th)/He data (n = 64 new, 24 published individual analyses) record hematite mineralization events ca. 0.8 Ma to 0.4 Ma at <1.5 km depth. We suggest these hematite faults formed via fluid overpressure, and then hematite localized repeated subseismic slip, creating zones of shallow off-fault damage as far as 4 km orthogonal to the trace of the southern San Andreas fault. Distributed hematite slip surfaces develop by, and then accommodate, transient slow slip, potentially dampening or distributing earthquake energy in shallow continental faults.