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Abstract Natural materials are highly organized, frequently possessing intricate and sophisticated hierarchical structures from which superior properties emerge. In the wake of biomimicry, there is a growing interest in designing architected materials in the laboratory as such structures could enable myriad functionalities in engineering. Yet, their fabrication remains challenging despite recent progress in additive manufacturing. In particular, soft materials are typically poorly suited to form the requisite structures consisting of regular geometries. Here, a new frugal methodology is reported to fabricate pixelated soft materials. This approach is conceptually analogous to the watershed transform used in image analysis and allows the passive assembly of complex geometries through the capillary‐mediated flow of curable elastomers in confined geometries. Emerging from sources distributed across a Hele–Shaw cell consisting of two parallel flat plates separated by an infinitesimally small gap, these flows eventually meet at the “dividing lines” thereby forming Voronoi tesselations. After curing is complete, these structures turn into composite elastic sheets. Rationalizing the fluid mechanics at play allows the structural geometry of the newly formed sheets to be tailored and thereby their local material properties to be tuned. 

In fiber spinning of photopolymers, surface tension limits the diameter of the fiber that can be produced due to the Rayleigh–Plateau instability. Submerging a pre-fiber jet in a miscible environment liberates the system from capillary effects, thus allowing the jet to be stretched into thin threads without instability. In this work, we systematically investigated a spinning method using miscible liquids, called jet-assisted wet spinning (JAWS), where stretching is achieved by a nearby submerged liquid jet. The diameter of the pre-fiber jet is a function of its flow rate and position relative to the assisting submerged liquid jet. A particular case where the main jet is modeled as the Landau–Squire jet is used to demonstrate the tracer-like thinning behavior of the pre-fiber jet. Experiments show that buoyancy has a significant impact on the pre-fiber jet diameter because of its influence on the entrainment trajectory. Overall, our results demonstrate the potential for the parallelization of JAWS for high-throughput fiber production. 

Droplet crystals can form when marrying 3D printing to fluidic instabilities.