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Abstract Hybrid magnonic systems are a newcomer for pursuing coherent information processing owing to their rich quantum engineering functionalities. One prototypical example is hybrid magnonics in antiferromagnets with an easy-plane anisotropy that resembles a quantum-mechanically mixed two-level spin system through the coupling of acoustic and optical magnons. Generally, the coupling between these orthogonal modes is forbidden due to their opposite parity. Here we show that the Dzyaloshinskii–Moriya-Interaction (DMI), a chiral antisymmetric interaction that occurs in magnetic systems with low symmetry, can lift this restriction. We report that layered hybrid perovskite antiferromagnets with an interlayer DMI can lead to a strong intrinsic magnon-magnon coupling strength up to 0.24 GHz, which is four times greater than the dissipation rates of the acoustic/optical modes. Our work shows that the DMI in these hybrid antiferromagnets holds promise for leveraging magnon-magnon coupling by harnessing symmetry breaking in a highly tunable, solution-processable layered magnetic platform.more » « less
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In this work, we theoretically study the switching and oscillation dynamics in strained non-collinear antiferromagnet (AFM) Mn3X (X = Sn, Ge, etc.). Using the perturbation theory, we identify three separable dynamic modes—one uniform and two optical modes, for which we analytically derive the oscillation frequencies and effective damping. We also establish a compact, vector equation for describing the dynamics of the uniform mode, which is in analogy to the conventional Landau–Lifshitz–Gilbert (LLG) equation for ferromagnet but captures the unique features of the cluster octuple moment. Extending our model to include spatial inhomogeneity, we are able to describe the excitations of dissipative spin wave and spin superfluidity state in the non-collinear AFM. Furthermore, we carry out numerical simulations based on coupled LLG equations to verify the analytical results, where good agreements are reached. Our treatment with the perturbative approach provides a systematic tool for studying the dynamics of non-collinear AFM and is generalizable to other magnetic systems in which the Hamiltonian can be expressed in a hierarchy of energy scales.more » « less
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Recently discovered magnetic Weyl semimetals (MWSM), with enhanced Berry curvature stemming from the topology of their electronic band structure, have gained much interest for spintronics applications. In this category, Co2MnGa, a room temperature ferromagnetic Heusler alloy, has garnered special interest as a promising material for topologically driven spintronic applications. However, until now, the structural-order dependence of spin current generation efficiency through the spin Hall effect has not been fully explored in this material. In this paper, we study the evolution of magnetic and transport properties of Co2MnGa thin films from the chemically disordered B2 to ordered L21 phase. We also report on the change in spin generation efficiency across these different phases, using heterostructures of Co2MnGa and ferrimagnet CoxTb1−x with perpendicular magnetic anisotropy. We measured large spin Hall angles in both the B2 and L21 phases, and within our experimental limits, we did not observe the advantage brought by the MWSM ordering in generating a strong spin Hall angle over the disordered phases, which suggests more complicated mechanisms over the intrinsic, Weyl-band structure-determined spin Hall effect in these material stacks.more » « less
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