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Abstract Manipulating the topological properties of spin textures in magnetic materials is of great interest due to the rich physics and promising technological applications of these materials in advanced electronic devices. A spin texture with desired topological properties can be created by magnetic monopole injection, resulting in topological transitions involving changes in the topological charge. Therefore, controlling magnetic monopole injection has paramount importance for obtaining the desired spin textures but has not yet been reported. Here, we report the use of reliably manipulated magnetic monopole injection in the topological transition from stripe domains to skyrmions in an Fe/Gd multilayer. An easily tunable in-plane magnetic field applied to an Fe/Gd multilayer plays a key role in the magnetic monopole injection by modulating the local exchange energy. Our findings facilitate the efficient management of topological transitions by providing an important method for controlling magnetic monopole injection.more » « less
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Abstract The presence of multiple competing periodicities may result in a system to go through states with modulated periodicities, an example of which is the self-similar staircase-like structure called the Devil’s Staircase. Herein we report on a novel staircase structure of domain periodicity in an amorphous and centrosymmetric Fe/Gd magnetic thin film system wherein the reciprocal space wavevectorQdue to the ordered stripe domains does not evolve continuously, rather exhibits a staircase structure. Resonant X-ray scattering experiments show jumps in the periodicity of the stripe domains as a function of an external magnetic field. When resolved in components, the length-scale step change along Qxwas found to be an integral multiple of a minimum step height of 7 nm, which resembles closely to the exchange length of the system. Modeling the magnetic texture in the Fe/Gd system as an achiral spin arrangement, we have been able to reproduce the steps in the magnetization using a Landau-Lifshitz spin dynamics calculation. Our results indicate that anisotropy and not the dipolar interaction is the dominant cause for the staircase pattern, thereby revealing the effect of achiral magnetism.more » « less
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Abstract Magnetic skyrmions exhibit unique, technologically relevant pseudo‐particle behaviors which arise from their topological protection, including well‐defined, 3D dynamic modes that occur at microwave frequencies. During dynamic excitation, spin waves are ejected into the interstitial regions between skyrmions, creating the magnetic equivalent of a turbulent sea. However, since the spin waves in these systems have a well‐defined length scale, and the skyrmions are on an ordered lattice, ordered structures from spin‐wave interference can precipitate from the chaos. This work uses small‐angle neutron scattering (SANS) to capture the dynamics in hybrid skyrmions and investigate the spin‐wave structure. Performing simultaneous ferromagnetic resonance and SANS, the diffraction pattern shows a large increase in low‐angle scattering intensity, which is present only in the resonance condition. This scattering pattern is best fit using a mass fractal model, which suggests the spin waves form a long‐range fractal network. The fractal structure is constructed of fundamental units with a size that encodes the spin‐wave emissions and are constrained by the skyrmion lattice. These results offer critical insights into the nanoscale dynamics of skyrmions, identify a new dynamic spin‐wave fractal structure, and demonstrate SANS as a unique tool to probe high‐speed dynamics.more » « less
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Abstract Herein, the experimental observation of micrometer‐scale magnetic skyrmions at room temperature in several Pt/Co‐based thin film heterostructures designed to possess low exchange stiffness, perpendicular magnetic anisotropy, and a modest interfacial Dzyaloshinskii–Moriya interaction (iDMI) is reported. It is found both experimentally and by micromagnetic and analytic modeling that a low exchange stiffness and modest iDMI eliminates the energetic penalty associated with forming domain walls in thin films. When the domain wall energy density approaches negative values, the remanent morphology transitions from a uniform state to labyrinthine stripes. A low exchange stiffness, indicated by a sub‐400 K Curie temperature, is achieved in Pt/Co, Pt/Co/Ni, and Pt/Co/Ni/Re structures by reducing the Co thickness to the ultrathin limit (<0.3 nm). Similar effects occur in thicker Pt/Co/NixCu1−xstructures when the Ni layer is alloyed with Cu. At this transition in domain morphology, skyrmion phases are stabilized by small (<1 mT), perpendicular magnetic fields, and skyrmion motion in response to spin–orbit torque is observed. While the temperature and thickness‐induced morphological phase transitions observed are similar to the well‐studied spin reorientation transition that occurs in the ultrathin limit, the underlying energy balances are substantially modified by the presence of an iDMI.more » « less
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