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Free, publicly-accessible full text available April 1, 2024
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McCluskey, Matthew D. ; Pansegrau, Christopher ; Ahmed, Syeed E. ; Santillan, Macarena ; Jesenovec, Jani ; McCloy, John S. ( , Proc. SPIE)Teherani, Ferechteh H. ; Rogers, David J. (Ed.)
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Pansegrau, Christopher ; McCluskey, Matthew D. ( , Journal of Applied Physics)
Annealed bulk crystals of barium titanate (BaTiO3) exhibit persistent photoconductivity (PPC) at room temperature. Samples were annealed in a flowing gas of humid argon and hydrogen, with a higher flow rate corresponding to larger PPC. When exposed to sub-bandgap light, a broad infrared (IR) absorption peak appears at 5000 cm−1(2 μm), attributed to polaronic or free-carrier absorption from electrons in the conduction band. Along with the increased IR absorption, electrical resistance is reduced by a factor of approximately two. The threshold photon energy for PPC is 2.9 eV, similar to the case of SrTiO3. This similarity suggests that the mechanisms are similar: an electron in substitutional hydrogen (HO) is photoexcited into the conduction band, causing the proton to leave the oxygen vacancy and attach to a host oxygen atom. The barrier to recover to the ground state is large such that PPC persists at room temperature.
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Ahmed, Syeed E. ; Poole, Violet M. ; Igo, John ; Gu, Yi ; McCluskey, Matthew D. ( , Journal of Vacuum Science & Technology A)