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Whenever the elastic energy of a solid depends on magnetic field, there is a magnetostrictive response. Field-linear magnetostriction implies piezo- magnetism and vice versa. Here, we show that Mn3Sn, a non-collinear anti- ferromanget with Weyl nodes, hosts a large and almost perfectly linear magnetostriction even at room temperature. The longitudinal and transverse magnetostriction, with opposite signs and similar amplitude are restricted to the kagome planes and the out-of-plane response is negligibly small. By studying four different samples with different Mn:Sn ratios, we find a clear correlation between the linear magnetostriction, the spontaneous magneti- zation and the concentration of Sn vacancies. The recently reported piezo- magnetic data fits in our picture. We show that linear magnetostriction and piezomagnetism are both driven by the field-induced in-plane twist of spins. A quantitative account of the experimental data requires the distortion of the spin texture by Sn vacancies. We find that the field-induced domain nucleation within the hysteresis loop corresponds to a phase transition. Within the hys- teresis loop, a concomitant mesoscopic modulation of local strain and spin twist angles, leading to twisto-magnetic stripes, arises as a result of the com- petition between elastic and magnetic energies.more » « lessFree, publicly-accessible full text available December 1, 2025
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Inspired by the recent work by Delacretaz et. al. [Phys. Rev. Res. 4, 033131 (2022)], we rigorously derive an exact and simple method to bosonize a non-interacting fermionic system with a Fermi surface starting from a microscopic Hamiltonian. In the long-wavelength limit, we show that the derived bosonized action is exactly equivalent to the action obtained by Delacretaz et. al. In addition, we propose diagrammatic rules to evaluate correlation functions using our bosonized theory and demonstrate these rules by calculating the three- and four-point density correlation functions. We also consider a general density-density interaction and show that the simplest approximation in our bosonic theory is identical to RPA results.more » « less
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Abstract Magnetic order in most materials occurs when magnetic ions with finite moments arrange in a particular pattern below the ordering temperature. Intriguingly, if the crystal electric field (CEF) effect results in a spin-singlet ground state, a magnetic order can still occur due to the exchange interactions between neighboring ions admixing the excited CEF levels. The magnetic excitations in such a state are spin excitons generally dispersionless in reciprocal space. Here we use neutron scattering to study stoichiometric Ni 2 Mo 3 O 8 , where Ni 2+ ions form a bipartite honeycomb lattice comprised of two triangular lattices, with ions subject to the tetrahedral and octahedral crystalline environment, respectively. We find that in both types of ions, the CEF excitations have nonmagnetic singlet ground states, yet the material has magnetic order. Furthermore, CEF spin excitons from the tetrahedral sites form a dispersive diffusive pattern around the Brillouin zone boundary, likely due to spin entanglement and geometric frustrations.more » « less
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We present experimental and theoretical evidence of novel bound state formation in the low transverse field or- dered phase of the quasi-one-dimensional Ising-like material CoNb2O6. High-resolution single-crystal inelastic neutron scattering measurements observe that small transverse fields lead to a breakup of the spectrum into three parts, each evolving very differently upon increasing field. This can be naturally understood starting from the excitations of the ordered phase of the transverse field Ising model, domain wall quasiparticles (solitons). Here, the transverse field and a staggered off-diagonal exchange create one-soliton hopping terms with opposite signs. We show that this leads to a rich spectrum and a special field, when the strengths of the off-diagonal exchange and transverse field match, at which solitons become localized; the highest field investigated is very close to this special regime. We solve this case analytically and find three two-soliton continua, along with three novel bound states. Perturbing away from this novel localized limit, we find very good qualitative agreement with the experimental data. We also present calculations using exact diagonalization of a recently refined Hamiltonian model for CoNb2O6 and using diagonalization of the two-soliton subspace, both of which provide a quantitative agreement with the observed spectrum. The theoretical models qualitatively and quantitatively capture a variety of nontrivial features in the observed spectrum, providing insight into the underlying physics of bound state formation.more » « less