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Ultrasound computed tomography (USCT) is one of the advanced imaging techniques used in structural health monitoring (SHM) and medical imaging due to its relatively low-cost, rapid data acquisition process. The time-domain full waveform inversion (TDFWI) method, an iterative inversion approach, has shown great promise in USCT. However, such an iterative process can be very time-consuming and computationally expensive but can be greatly accelerated by integrating an AI-based approach (e.g., convolution neural network (CNN)). Once trained, the CNN model takes low-iteration TDFWI images as input and instantaneously predicts material property distribution within the scanned region. Nevertheless, the quality of the reconstruction with the current CNN degrades with the increased complexity of material distributions. Another challenge is the availability of enough experimental data and, in some cases, even synthetic surrogate data. To alleviate these issues, this paper details a systematic study of the enhancement effect of a 2D CNN (U-Net) by improving the quality with limited training data. To achieve this, different augmentation schemes (flipping and mixing existing data) were implemented to increase the amount and complexity of the training datasets without generating a substantial number of samples. The objective was to evaluate the enhancement effect of these augmentation techniques on the performance of the U-Net model at FWI iterations. A thousand numerically built samples with acoustic material properties are used to construct multiple datasets from different FWI iterations. A parallelized, high-performance computing (HPC) based framework has been created to rapidly generate the training data. The prediction results were compared against the ground truth images using standard matrices, such as the structural similarity index measure (SSIM) and average mean square error (MSE). The results show that the increased number of samples from augmentations improves shape imaging of the complex regions even with a low iteration FWI training data.