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Abstract Semiconductor excitations can hybridize with cavity photons to form exciton-polaritons (EPs) with remarkable properties, including light-like energy flow combined with matter-like interactions. To fully harness these properties, EPs must retain ballistic, coherent transport despite matter-mediated interactions with lattice phonons. Here we develop a nonlinear momentum-resolved optical approach that directly images EPs in real space on femtosecond scales in a range of polaritonic architectures. We focus our analysis on EP propagation in layered halide perovskite microcavities. We reveal that EP–phonon interactions lead to a large renormalization of EP velocities at high excitonic fractions at room temperature. Despite these strong EP–phonon interactions, ballistic transport is maintained for up to half-exciton EPs, in agreement with quantum simulations of dynamic disorder shielding through light-matter hybridization. Above 50% excitonic character, rapid decoherence leads to diffusive transport. Our work provides a general framework to precisely balance EP coherence, velocity, and nonlinear interactions.more » « less
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Xu, Ding; Peng, Zhi Hao; Trovatello, Chiara; Cheng, Shan-Wen; Xu, Xinyi; Sternbach, Aaron; Basov, D N; Schuck, P James; Delor, Milan (, Nature Nanotechnology)Free, publicly-accessible full text available March 1, 2026
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Lee, Inki; Melton, Sarah R; Xu, Ding; Delor, Milan (, Journal of the American Chemical Society)
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Mandal, Arkajit; Xu, Ding; Mahajan, Ankit; Lee, Joonho; Delor, Milan; Reichman, David R. (, Nano Letters)
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