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Award ID contains: 2210186

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  1. Topological semimetals with massless Dirac and Weyl fermions represent the forefront of quantum materials research. In two dimensions, a peculiar class of fermions that are massless in one direction and massive in the perpendicular direction was predicted 16 years ago. These highly exotic quasiparticles—the semi-Dirac fermions—ignited intense theoretical and experimental interest but remain undetected. Using magneto-optical spectroscopy, we demonstrate the defining feature of semi-Dirac fermions— B 2 / 3 scaling of Landau levels—in a prototypical nodal-line metal ZrSiS. In topological metals, including ZrSiS, nodal lines extend the band degeneracies from isolated points to lines, loops, or even chains in the momentum space. With calculations and theoretical modeling, we pinpoint the observed semi-Dirac spectrum to the crossing points of nodal lines in ZrSiS. Crossing nodal lines exhibit a continuum absorption spectrum but with singularities that scale as B 2 / 3 at the crossing. Our work sheds light on the hidden quasiparticles emerging from the intricate topology of crossing nodal lines and highlights the potential to explore quantum geometry with linear optical responses. Published by the American Physical Society2024 
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    Free, publicly-accessible full text available December 1, 2025
  2. We present a basic framework for modeling collective mode effects in photocurrent measurements performed on two-dimensional materials using nano-optical scanned probes. We consider photothermal, photovoltaic, and bolometric contributions to the photocurrent. We show that any one of these can dominate depending on frequency, temperature, applied bias, and sample geometry. Our model is able to account for periodic spatial oscillations (fringes) of the photocurrent observed near sample edges or inhomogeneities. For the case of a non-absorbing substrate, we find a direct relation between the spectra measured by the photocurrent nanoscopy and its parental scanning technique near-field optical microscopy. 
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