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Abstract The increasing demand for concrete in construction presents challenges such as pollution, high energy consumption, and complex structural requirements. Three‐dimensional printing (3DP) offers a promising solution by eliminating formwork, reducing waste, and enabling intricate geometries. Predicting the strength of 3D‐printed fiber‐reinforced concrete (3DP‐FRC) remains challenging due to the nonlinear nature of neural networks and uncertainty in optimizing key parameters. In this study, we developed machine learning models using five metaheuristic algorithms—arithmetic optimization algorithm, African Vulture Optimization Algorithm, flow direction algorithm, generalized normal distribution optimization, and Mountain Gazelle Optimizer—to optimize the weights and biases in a feed‐forward backpropagation network. Among all the algorithms, MGO demonstrated the best performance. To address data limitations, a data augmentation method combining Kernel density estimation and Wasserstein generative adversarial networks is employed. Sensitivity analysis using SHapley Additive exPlanations (SHAP) identifies the most influential input parameters. The proposed MGO‐ANN model enhances predictive accuracy, reducing the need for extensive laboratory testing. Additionally, a user‐friendly graphical user interface is developed to facilitate practical applications in estimating 3DP‐FRC flexural strength.