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AbstractThis article presents an overview of the current status and future prospects of integrated nonlinear photonics in the long-wave infrared (LWIR) spectrum, spanning 6 to 14 μm. This range is well-suited for applications such as chemical identification, environmental monitoring, surveillance, search and rescue, and night vision. Nevertheless, the advancement of a mature, low-loss chip-level platform for the LWIR remains in its infancy. We examine the materials growth techniques, and fabrication methods associated with integrated nonlinear photonics in the LWIR, highlighting promising platforms like chalcogenide glass, single-crystalline diamond, Ge/SiGe, and III–V compounds. Furthermore, we explore loss mechanisms, dispersion engineering, nonlinear generation of broadband supercontinuum and frequency combs, and device performance, encompassing photodetectors and modulators. Lastly, we propose a roadmap for the future development of integrated nonlinear photonics in the LWIR. Graphic Abstract 

Abstract The longwave infrared (LWIR) range, which spans from 6 µm to 14 µm, is appealing for sensing due to strong molecular fingerprints in this range. However, the limited availability of low-loss materials that can provide higher-index waveguiding and lower-index cladding in the LWIR range presents challenges for integrated photonics. In this work, we introduce a low-loss germanium-on-zinc selenide (GOZ) platform that could serve as a versatile platform for nanophotonics in the LWIR. By bonding high-quality thin-film germanium (Ge) to a zinc selenide (ZnSe) substrate, we demonstrate transparency from 2 µm to 14 µm and optical losses of just 1 cm⁻¹at 7.8 µm. Our results demonstrate that hybrid photonic platforms could be invaluable for overcoming the losses of epitaxially grown materials and could enable a wide range of future quantum and nonlinear photonics. 

Abstract The longwave infrared (LWIR) region of the spectrum spans 8 to 14 μm and enables high-performance sensing and imaging for detection, ranging, and monitoring. Chip-scale LWIR photonics has enormous potential for real-time environmental monitoring, explosive detection, and biomedicine. However, realizing technologies such as precision sensors and broadband frequency combs requires ultra low-loss and low-dispersion components, which have so far remained elusive in this regime. Here, we use native germanium to demonstrate the first high-quality microresonators in the LWIR. These microresonators are coupled to partially-suspended Ge waveguides on a separate glass chip, allowing for the first unambiguous measurements of isolated linewidths. At 8 μm, we measured losses of 0.5 dB/cm and intrinsic quality (Q) factors of 2.5 × 10⁵, nearly two orders of magnitude higher than prior LWIR resonators. Our work portends the development of novel sensing and nonlinear photonics in the LWIR regime. 

Quantum cascade lasers (QCLs) have emerged as promising candidates for generating chip-scale frequency combs in mid-infrared and terahertz wavelengths. In this work, we demonstrate frequency comb formation in ring terahertz QCLs using the injection of light from a distributed feedback (DFB) laser. The DFB design frequency is chosen to match the modes of the ring cavity (near 3.3 THz), and light from the DFB is injected into the ring QCL via a bus waveguide. By controlling the power and frequency of the optical injection, we show that combs can be selectively formed and controlled in the ring cavity. Numerical modeling suggests that this comb is primarily frequency-modulated in character, with the injection serving to trigger comb formation. We also show that the ring can be used as a filter to control the output of the DFB QCL, potentially being of interest in terahertz photonic integrated circuits. Our work demonstrates that waveguide couplers are a compelling approach for injecting and extracting radiation from ring terahertz combs and offer exciting possibilities for the generation of new comb states in terahertz, such as frequency-modulated waves, solitons, and more. 

Frequency-modulated (FM) combs with a linearly-chirped frequency and nearly constant intensity occur naturally in certain laser systems; they can be most succinctly described by a nonlinear Schrödinger equation with a phase potential. In this work, we perform a comprehensive analytical study of FM combs in order to calculate their salient properties. We develop a general procedure that allows mean-field theories to be constructed for arbitrary sets of master equations, and as an example consider the case of reflective defects. We derive an expression for the FM chirp of arbitrary Fabry-Perot cavities—important for most realistic lasers—and use perturbation theory to show how they are affected by finite gain bandwidth and linewidth enhancment in fast gain media. Lastly, we show that an eigenvalue formulation of the laser’s dynamics can be useful for characterizing all of the stable states of the laser: the fundamental comb, the continuous-wave solution, and the harmonic states.