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Photoinduced Electron Transfer in an Ethyne Bridged Donor-Acceptor Complex Depends Strongly on Torsion Angle

Mendis, Kasun C. ; Li, Xiao ; Valdiviezo, Jesús ; Banziger, Susannah D. ; Zhang, Peng ; Ren, Tong ; Beratan, David N. ; Rubtsov, Igor V. ( May 2021 , International Conference on Time Resolved Vibrational Spectroscopy)
Kubarych, Kevin ; Ogilvie, Jennifer (Ed.)
Photoinduced electron transfer (ET) between electron donor (dimethylaniline) and acceptor (N-isopropyl-1,8-napthalimide) covalently linked by ethyne bridge is investigated by a mid-IR transient absorption spectroscopy and TD-DFT computations. We found that electronic and vibrational properties of the complex, including ET rate, depends strongly on the D-A torsion angle.
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