The field of (U-Th)/He geochronology and thermochronology has grown enormously over the past ∼25 years. The tool is applicable across much of geologic time, new (U-Th)/He chronometers are under continuous development, and the method is used in a diverse array of studies. Consequently, the technique has a rapidly expanding user base, and new labs are being established worldwide. This presents both opportunities and challenges. Currently there are no universally agreedupon protocols for reporting measured (U-Th)/He data or data derivatives. Nor are there standardized practices for reporting He diffusion kinetic, 4He/3He, or continuous ramped heating data. Approaches for reporting uncertainties associated with all types of data also vary widely. Here, we address these issues. We review the fundamentals of the methods, the types of materials that can be dated, how data are acquired, the process and choices associated with data reduction, and make recommendations for data and uncertainty reporting. We advocate that both the primary measured and derived data be reported, along with statements of assumptions, appropriate references, and clear descriptions of the methods used to compute derived data from measured values. The adoption of more comprehensive and uniform approaches to data and uncertainty reporting will enable data to be re-reduced in the future with different interpretative contexts and data reduction methods, and will facilitate inter-comparison of data sets generated by different laboratories. Together, this will enhance the value, cross-disciplinary use, reliability, and ongoing development of (U-Th)/He chronology.
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Characterization of helium release from apatite by continuous ramped heating
Knowledge of the kinetic behavior of He in apatite and other U- and Th-bearing minerals comes largely from detailed step-heating experiments, yet such experiments are time consuming and are rarely performed during routine thermochronological studies using the U-Th/He method. We propose a new analytical method for measuring both the bulk 4He abundance and the kinetics of He release in apatite. Using this method He is extracted from samples by continuous heating using a ramped temperature schedule under static vacuum conditions, and the evolved He is measured periodically as it accumulates in the extraction system. Continuous ramped heating (CRH) experiments can be conducted using instrumentation available in most noble-gas ther- mochronology labs but require particular attention to temperature control, measurement linearity and dynamic range, and suppression of active gases co-evolved with He. CRH experiments require little more time than conventional single-step heating measurements but yield a detailed record of He release not provided by con- ventional methods. Kinetic parameters for He diffusion in Durango apatite derived from continuous heating data agree well with those obtained from published step-heating studies. The continuous record of He release ob- tained from CRH experiments also provides important information about the siting of He and the presence of multiple He components in apatite, some of which may be responsible for anomalous U-Th/He ages and high age dispersion. As such the CRH method shows promise as a useful sample screening tool for apatite U-Th/He thermochronology.
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- Award ID(s):
- 1726350
- PAR ID:
- 10060776
- Date Published:
- Journal Name:
- Chemical geology
- Volume:
- 476
- ISSN:
- 0009-2541
- Page Range / eLocation ID:
- 223-232
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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