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1. Limits on the Rate of Conversion of Potential to Kinetic Energy in Quasigeostrophic Turbulence

   https://doi.org/10.3390/fluids7080276  

   Grooms, Ian (August 2022, Fluids)

   Flow configurations that maximize the instantaneous rate of conversion from potential to kinetic energy are sought using a combination of analytical and numerical methods. A hydrostatic model is briefly investigated, but the presence of unrealistic ageostrophic flow configurations renders the results unrealistic. In the quasigeostrophic (QG) model, flow configurations that locally optimize the conversion rate are found, but it remains unclear if these flow configurations produce the global maximum conversion rate. The difficulty is associated with the fact that in the QG model, the vertical velocity is a quadratic function of the QG streamfunction, which renders the conversion rate a cubic function of the QG streamfunction. For these locally maximal conversion rates, the rate of conversion depends on the horizontal length scale of the flow: for scales larger than the deformation radius, the maximal rates are small and decrease as the horizontal scale increases; for scales smaller than the deformation radius, the maximal conversion rate rises until it becomes comparable to the maximal rate at which potential energy can be extracted from the mean flow. 

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2. Theory of χ ⁽²⁾ -microresonator-based frequency conversion

   https://doi.org/10.1364/OL.427684  

   Zhao, Yun; Jang, Jae_K; Okawachi, Yoshitomo; Gaeta, Alexander_L (October 2021, Optics Letters)

   Microresonator-based platforms withnonlinearities have the potential to perform frequency conversion at high efficiencies and ultralow powers with small footprints. The standard doctrine for achieving high conversion efficiency in cavity-based devices requires “perfect matching,” that is, zero phase mismatch while all relevant frequencies are precisely at a cavity resonance, which is difficult to achieve in integrated platforms due to fabrication errors and limited tunabilities. In this Letter, we show that the violation of perfect matching does not necessitate a reduction in conversion efficiency. On the contrary, in many cases, mismatches should be intentionally introduced to improve the efficiency or tunability of conversion. We identify the universal conditions for maximizing the efficiency of cavity-based frequency conversion and show a straightforward approach to fully compensate for parasitic processes such as thermorefractive and photorefractive effects that, typically, can limit the conversion efficiency. We also show the design criteria that make these high-efficiency states stable against nonlinearity-induced instabilities. 

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3. Two‐Photon Up‐Conversion Photoluminescence Realized through Spatially Extended Gap States in Quasi‐2D Perovskite Films

   https://doi.org/10.1002/adma.201901240  

   Zhu, Xixiang; Xu, Hengxing; Liu, Yongtao; Zhang, Jia; Wang, Miaosheng; Ivanov, Ilia_N; Ovchinnikova, Olga_S; Hu, Bin (October 2019, Advanced Materials)

   Abstract A new approach to generate a two‐photon up‐conversion photoluminescence (PL) by directly exciting the gap states with continuous‐wave (CW) infrared photoexcitation in solution‐processing quasi‐2D perovskite films [(PEA)₂(MA)₄Pb₅Br₁₆withn= 5] is reported. Specifically, a visible PL peaked at 520 nm is observed with the quadratic power dependence by exciting the gap states with CW 980 nm laser excitation, indicating a two‐photon up‐conversion PL occurring in quasi‐2D perovskite films. Decreasing the gap states by reducing thenvalue leads to a dramatic decrease in the two‐photon up‐conversion PL signal. This confirms that the gap states are indeed responsible for generating the two‐photon up‐conversion PL in quasi‐2D perovskites. Furthermore, mechanical scratching indicates that the different‐n‐value nanoplates are essentially uniformly formed in the quasi‐2D perovskite films toward generating multi‐photon up‐conversion light emission. More importantly, the two‐photon up‐conversion PL is found to be sensitive to an external magnetic field, indicating that the gap states are essentially formed as spatially extended states ready for multi‐photon excitation. Polarization‐dependent up‐conversion PL studies reveal that the gap states experience the orbit–orbit interaction through Coulomb polarization to form spatially extended states toward developing multi‐photon up‐conversion light emission in quasi‐2D perovskites. 

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4. Back-conversion suppressed parametric frequency conversion for ultrawide bandwidth and ultrahigh efficiency devices

   https://doi.org/10.1117/12.2548361  

   Moses, Jeffrey; Flemens, Noah; Ding, Xiaoyue; Schunemann, Peter G.; Schepler, Kenneth L. (March 2020, SPIE LASE, 2020, San Francisco, California, United States)

   For as widely used a tool as nonlinear optical frequency conversion is for both science and industry, it remains widely limited in eciency and bandwidth (and ultimately also in cost) due to the fundamental problem of backconversion in the nonlinear evolution dynamics. This review paper covers new developments and capabilities in frequency conversion devices, including optical up- and down-converters and ampli ers, based on nonlinear evolution dynamics in which back-conversion is suppressed. One such approach is adiabatic frequency conversion, in which the dynamics of rapid adiabatic passage replace the regular cyclic conversion evolution in phase-matched sum- and dierence-frequency generation. This approach has enabled devices far surpassing the conventional eciency-bandwidth trade-o. For example, in chirped quasi-phase matched quadratic crystals, microjouleenergy single-cycle mid-infrared pulses were generated with arbitrary pulse shaping capability, presenting a source with unique features for nonlinear spectroscopy and strong- eld physics applications. We review new developments in the use of optical bers as a cubic nonlinear platform for the same concept, utilizing a tapered core diameter or a pressure gradient to allow up- and down-conversion with ultra-wide bandwidth and high eciency. We also review a newly introduced concept for high eciency optical parametric ampli cation, via a novel approach for suppressing back-conversion in optical parametric ampli cation by simultaneously phasematching the idler wave for second harmonic generation. Keywords: Adiabatic wave mixing, ecient optical parametric ampli cation, octave-spanning 

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5. Electrospun Cadmium Selenide Nanoparticles-Loaded Cellulose Acetate Fibers for Solar Thermal Application

   https://doi.org/10.3390/nano10071329  

   Angel, Nicole; Vijayaraghavan, S. N.; Yan, Feng; Kong, Lingyan (July 2020, Nanomaterials)

   null (Ed.)

   Solar thermal techniques provide a promising method for the direct conversion of solar energy to thermal energy for applications, such as water desalination. To effectively realize the optimal potential of solar thermal conversion, it is desirable to construct an assembly with localized heating. Specifically, photoactive semiconducting nanoparticles, when utilized as independent light absorbers, have successfully demonstrated the ability to increase solar vapor efficiency. Additionally, bio-based fibers have shown low thermal conductive photocorrosion. In this work, cellulose acetate (CA) fibers were loaded with cadmium selenide (CdSe) nanoparticles to be employed for solar thermal conversion and then subsequently evaluated for both their resulting morphology and conversion potential and efficiency. Electrospinning was employed to fabricate the CdSe-loaded CA fibers by adjusting the CA/CdSe ratio for increased solar conversion efficiency. The microstructural and chemical composition of the CdSe-loaded CA fibers were characterized. Additionally, the optical sunlight absorption performance was evaluated, and it was demonstrated that the CdSe nanoparticles-loaded CA fibers have the potential to significantly improve solar energy absorption. The photothermal conversion under 1 sun (100 mW/cm2) demonstrated that the CdSe nanoparticles could increase the temperature up to 43 °C. The CdSe-loaded CA fibers were shown as a feasible and promising hybrid material for achieving efficient solar thermal conversion. 

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