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1. Designer pair statistics of disordered many-particle systems with novel properties

   https://doi.org/10.1063/5.0189769  

   Wang, Haina; Torquato, Salvatore (January 2024, The Journal of Chemical Physics)

   The knowledge of exact analytical functional forms for the pair correlation function g2(r) and its corresponding structure factor S(k) of disordered many-particle systems is limited. For fundamental and practical reasons, it is highly desirable to add to the existing database of analytical functional forms for such pair statistics. Here, we design a plethora of such pair functions in direct and Fourier spaces across the first three Euclidean space dimensions that are realizable by diverse many-particle systems with varying degrees of correlated disorder across length scales, spanning a wide spectrum of hyperuniform, typical nonhyperuniform, and antihyperuniform ones. This is accomplished by utilizing an efficient inverse algorithm that determines equilibrium states with up to pair interactions at positive temperatures that precisely match targeted forms for both g2(r) and S(k). Among other results, we realize an example with the strongest hyperuniform property among known positive-temperature equilibrium states, critical-point systems (implying unusual 1D systems with phase transitions) that are not in the Ising universality class, systems that attain self-similar pair statistics under Fourier transformation, and an experimentally feasible polymer model. We show that our pair functions enable one to achieve many-particle systems with a wide range of translational order and self-diffusion coefficients D, which are inversely related to one another. One can design other realizable pair statistics via linear combinations of our functions or by applying our inverse procedure to other desirable functional forms. Our approach facilitates the inverse design of materials with desirable physical and chemical properties by tuning their pair statistics. 

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2. Local order metrics for many-particle systems across length scales

   https://doi.org/10.1103/PhysRevResearch.6.033262  

   Maher, Charles Emmett; Torquato, Salvatore (September 2024, Physical Review Research)

   Formulating order metrics that sensitively quantify the degree of order/disorder in many-particle systems in $d$-dimensional Euclidean space ${\mathbb{R}}^d$across length scales is an outstanding challenge in physics, chemistry, and materials science. Since an infinite set of $n$-particle correlation functions is required to fully characterize a system, one must settle for a reduced set of structural information, in practice. We initiate a program to use the local number variance ${\sigma }_N^2\left(R\right)$associated with a spherical sampling window of radius $R$(which encodes pair correlations) and an integral measure derived from it ${\mathrm{\Sigma }}_N(R_i,R_j)$that depends on two specified radial distances $R_i$and $R_j$. Across the first three space dimensions ( $d=1,2,3$), we find these metrics can sensitively describe and categorize the degree of order/disorder of 41 different models of antihyperuniform, nonhyperuniform, disordered hyperuniform, and ordered hyperuniform many-particle systems at a specified length scale $R$. Using our local variance metrics, we demonstrate the importance of assessing order/disorder with respect to a specific value of $R$. These local order metrics could also aid in the inverse design of structures with prescribed length-scale-specific degrees of order/disorder that yield desired physical properties. In future work, it would be fruitful to explore the use of higher-order moments of the number of points within a spherical window of radius $R$[S. Torquato , ] to devise even more sensitive order metrics. Published by the American Physical Society2024 

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3. Screening the Coulomb interaction leads to a prethermal regime in two-dimensional bad conductors

   https://doi.org/10.1038/s41467-023-42778-2  

   Stanley, L. J.; Lin, Ping V.; Jaroszyński, J.; Popović, Dragana (November 2023, Nature Communications)

   Abstract The absence of thermalization in certain isolated many-body systems is of great fundamental interest. Many-body localization (MBL) is a widely studied mechanism for thermalization to fail in strongly disordered quantum systems, but it is still not understood precisely how the range of interactions affects the dynamical behavior and the existence of MBL, especially in dimensionsD > 1. By investigating nonequilibrium dynamics in strongly disorderedD = 2 electron systems with power-law interactions ∝ 1/r^αand poor coupling to a thermal bath, here we observe MBL-like, prethermal dynamics forα = 3. In contrast, forα = 1, the system thermalizes, although the dynamics is glassy. Our results provide important insights for theory, especially since we obtained them on systems that are much closer to the thermodynamic limit than synthetic quantum systems employed in previous studies of MBL. Thus, our work is a key step towards further studies of ergodicity breaking and quantum entanglement in real materials. 

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4. Long-time properties of generic Floquet systems are approximately periodic with the driving period

   https://doi.org/10.1088/1367-2630/ad5eb1  

   Huang_黄溢辰, Yichen (July 2024, New Journal of Physics)

   Abstract A Floquet quantum system is governed by a Hamiltonian that is periodic in time. Consider the space of piecewise time-independent Floquet systems with (geometrically) local interactions. We prove that for all but a measure zero set of systems in this space, starting from a random product state, many properties (including expectation values of observables and the entanglement entropy of a macroscopically large subsystem) at long times are approximately periodic with the same period as the Hamiltonian. Thus, in almost every Floquet system of arbitrarily large but finite size, discrete time-crystalline behavior does not persist to strictly infinite time. 

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5. Reconnection and particle acceleration in three-dimensional current sheet evolution in moderately magnetized astrophysical pair plasma

   https://doi.org/10.1017/S0022377821001185  

   Werner, Gregory R.; Uzdensky, Dmitri A. (December 2021, Journal of Plasma Physics)

   Magnetic reconnection, a plasma process converting magnetic energy to particle kinetic energy, is often invoked to explain magnetic energy releases powering high-energy flares in astrophysical sources including pulsar wind nebulae and black hole jets. Reconnection is usually seen as the (essentially two-dimensional) nonlinear evolution of the tearing instability disrupting a thin current sheet. To test how this process operates in three dimensions, we conduct a comprehensive particle-in-cell simulation study comparing two- and three-dimensional evolution of long, thin current sheets in moderately magnetized, collisionless, relativistically hot electron–positron plasma, and find dramatic differences. We first systematically characterize this process in two dimensions, where classic, hierarchical plasmoid-chain reconnection determines energy release, and explore a wide range of initial configurations, guide magnetic field strengths and system sizes. We then show that three-dimensional (3-D) simulations of similar configurations exhibit a diversity of behaviours, including some where energy release is determined by the nonlinear relativistic drift-kink instability. Thus, 3-D current sheet evolution is not always fundamentally classical reconnection with perturbing 3-D effects but, rather, a complex interplay of multiple linear and nonlinear instabilities whose relative importance depends sensitively on the ambient plasma, minor configuration details and even stochastic events. It often yields slower but longer-lasting and ultimately greater magnetic energy release than in two dimensions. Intriguingly, non-thermal particle acceleration is astonishingly robust, depending on the upstream magnetization and guide field, but otherwise yielding similar particle energy spectra in two and three dimensions. Although the variety of underlying current sheet behaviours is interesting, the similarities in overall energy release and particle spectra may be more remarkable. 

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