Abstract Wildfires in the western United States are large sources of particulate matter, and the area burned by wildfires is predicted to increase in the future. Some particles released from wildfires can affect cloud formation by serving as ice‐nucleating particles (INPs). INPs have numerous impacts on cloud radiative properties and precipitation development. Wildfires are potentially important sources of INPs, as indicated from previous measurements, but their abundance in the free troposphere has not been quantified. The Western Wildfire Experiment for Cloud Chemistry, Aerosol Absorption, and Nitrogen campaign sampled free tropospheric immersion‐freezing INPs from smoke plumes near their source and downwind, along with widespread aged smoke. The results indicate an enhancement of INPs in smoke plumes relative to out‐of‐plume background air, but the magnitude of enhancement was both temperature and fire dependent. The majority of INPs were inferred to be predominately organic in composition with some contribution from biological sources at modest super cooling, and contributions from minerals at deeper super cooling. A fire involving primarily sagebrush shrub land and aspen forest fuels had the highest INP concentrations measured in the campaign, which is partially attributed to the INP characteristics of lofted, uncombusted plant material. Electron microscopy analysis of INPs also indicated tar balls present in this fire. Parameterization of the plume INP data on a per‐unit‐aerosol surface area basis confirmed that smoke is not an efficient source of INPs. Nevertheless, the high numbers of particles released from, and ubiquity of western US wildfires in summertime, regionally elevate INP concentrations in the free troposphere.
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The Impacts of Smoke Emitted from Boreal Forest Wildfires on the High Latitude Radiative Energy Budget—A Case Study of the 2002 Yakutsk Wildfires
We examine the 2002 Yakutsk wildfire event and simulate the impacts of smoke aerosols on local radiative energy budget, using the WRF-Chem-SMOKE model. When comparing satellite retrievals (the Surface Radiation Budget (SRB) dataset) with model simulations, we found that the agreement is generally good, except for the regions where the model predicts too few clouds or SRB misclassifies strong smoke plumes as clouds. We also found that the smoke-induced changes in upward shortwave fluxes at top of atmosphere (TOA) vary under different burning and meteorological conditions. In the first period of the fire season (9–12 August), smoke particles cause a warming effect around 3 W/m2, mainly through functioning as ice nuclei, which deplete the cloud water amount in the frontal system. At the beginning of the second period of the fire season (19–20 August), large amounts of pre-existing smoke particles cause a strong cooling effect of −8 W/m2. This is offset by the warming effect caused by relatively small amounts of cloud condensation nuclei increases, which promotes the rain formation and depletes the cloud water amount. After the cloud decks are well mixed with smoke plumes (21–22 August), the first indirect and direct effects of smoke together lead to a cooling of −10 W/m2. These results highlight the importance of meso-scale modeling efforts in estimating the smoke-induced changes in the radiative energy budget over high latitudes.
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- Award ID(s):
- 1637279
- PAR ID:
- 10112225
- Date Published:
- Journal Name:
- Atmosphere
- Volume:
- 9
- Issue:
- 10
- ISSN:
- 2073-4433
- Page Range / eLocation ID:
- 410
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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