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Abstract Andean glaciers have melted rapidly since the 1960s. While some melting is likely due to anthropogenic climate change driven by increasing greenhouse gases, deposition of light-absorbing particles such as black carbon (BC) may also play a role. We hypothesize that BC from fires in the Amazon Basin and elsewhere may be deposited on Andean glaciers, reducing the surface albedo and inducing further melting. Here we investigate the role of BC deposition on albedo changes in the Andes for 2014–2019 by combining atmospheric chemistry modeling with observations of BC in snow or ice at four mountain sites in Peru (Quelccaya, Huascarán, Yanapaccha, and Shallap) and at one site in Bolivia (Illimani). We find that annual mean ice BC concentrations simulated by the chemical transport model GEOS-Chem for 2014–2019 are roughly consistent with those observed at the site with the longest record, Huascarán, with overestimates of 15%–40%. Smoke from fires account for 20%–70% of total wet and dry deposition fluxes, depending on the site. The rest of BC deposited comes from fossil fuel combustion. Using a snow albedo model, we find that the annual mean radiative forcing from the deposition of smoke BC alone on snow ranges from +0.1 to +3.2 W m−2under clear-sky conditions, with corresponding average albedo reductions of 0.04%–1.1%. These ranges are dependent on site and snow grain size. This result implies a potentially significant climate impact of biomass burning in the Amazon on radiative forcing in the Andes.
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Influence of cloud microphysical processes on black carbon wet removal, global distributions, and radiative forcing
Abstract. Parameterizations that impact wet removal of black carbon (BC)remain uncertain in global climate models. In this study, we enhance thedefault wet deposition scheme for BC in the Community Earth System Model (CESM)to (a) add relevant physical processes that were not resolved in thedefault model and (b) facilitate understanding of the relative importanceof various cloud processes on BC distributions. We find that the enhancedscheme greatly improves model performance against HIPPO observationsrelative to the default scheme. We find that convection scavenging, aerosolactivation, ice nucleation, evaporation of rain or snow, and below-cloudscavenging dominate wet deposition of BC. BC conversion rates for processesrelated to in-cloud water–ice conversion (i.e., riming, the Bergeronprocess, and evaporation of cloud water sedimentation) are relativelysmaller, but have large seasonal variations. We also conduct sensitivitysimulations that turn off each cloud process one at a time to quantify theinfluence of cloud processes on BC distributions and radiative forcing.Convective scavenging is found to have the largest impact onBC concentrations at mid-altitudes over the tropics and even globally. Inaddition, BC is sensitive to all cloud processes over the NorthernHemisphere at high latitudes. As for BC vertical distributions, convectivescavenging greatly influences BC fractions at different altitudes.Suppressing BC droplet activation in clouds mainly decreases the fraction ofcolumn BC below 5 km, whereas suppressing BC ice nucleation increases thatabove 10 km. During wintertime, the Bergeron process also significantlyincreases BC concentrations at lower altitudes over the Arctic. Oursimulation yields a global BC burden of 85 Gg; corresponding directradiative forcing (DRF) of BC estimated using the Parallel Offline RadiativeTransfer (PORT) is 0.13 W m−2, much lower than previous studies. Therange of DRF derived from sensitivity simulations is large, 0.09–0.33 W m−2,corresponding to BC burdens varying from 73 to 151 Gg. Due todifferences in BC vertical distributions among each sensitivity simulation,fractional changes in DRF (relative to the baseline simulation) are alwayshigher than fractional changes in BC burdens; this occurs because relocating BCin the vertical influences the radiative forcing per BC mass. Our resultshighlight the influences of cloud microphysical processes on BC concentrationsand radiative forcing.
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- PAR ID:
- 10129213
- Date Published:
- Journal Name:
- Atmospheric Chemistry and Physics
- Volume:
- 19
- Issue:
- 3
- ISSN:
- 1680-7324
- Page Range / eLocation ID:
- 1587 to 1603
- Format(s):
- Medium: X
- Sponsoring Org:
- National Science Foundation
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- Free Publicly Accessible Full Text
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Accepted Manuscript1.0
- Journal Article:
- https://doi.org/10.5194/acp-19-1587-2019
